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02 Sep 12:11

Photoemission Spectroscopy Using Virtual Photons Emitted by Positron Sticking: A Complementary Probe for Top-Layer Surface Electronic Structures

by Alexander J. Fairchild, Varghese A. Chirayath, Randall W. Gladen, Ali R. Koymen, Alex H. Weiss, and Bernardo Barbiellini

Author(s): Alexander J. Fairchild, Varghese A. Chirayath, Randall W. Gladen, Ali R. Koymen, Alex H. Weiss, and Bernardo Barbiellini

Researchers have demonstrated a way of measuring the electronic states of a material’s surface while avoiding signal contaminations from deeper layers.


[Phys. Rev. Lett. 129, 106801] Published Mon Aug 29, 2022

24 Aug 09:52

[ASAP] A Capillary-Force-Assisted Transfer for Monolayer Transition-Metal-Dichalcogenide Crystals with High Utilization

by Jixing Cai, Huanjun Chen, Yanlin Ke, and Shaozhi Deng

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ACS Nano
DOI: 10.1021/acsnano.2c06147
17 Aug 08:23

[ASAP] Gate-Tunable Helical Currents in Commensurate Topological Insulator/Graphene Heterostructures

by Jonas Kiemle, Lukas Powalla, Katharina Polyudov, Lovish Gulati, Maanwinder Singh, Alexander W. Holleitner, Marko Burghard, and Christoph Kastl

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ACS Nano
DOI: 10.1021/acsnano.2c03370
15 Aug 07:43

[ASAP] Interlayer Coupling: An Additional Degree of Freedom in Two-Dimensional Materials

by Shenghai Pei, Zenghui Wang, and Juan Xia

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ACS Nano
DOI: 10.1021/acsnano.1c11498
15 Aug 07:41

Strain-Induced Exciton Hybridization in ${\mathrm{WS}}_{2}$ Monolayers Unveiled by Zeeman-Splitting Measurements

by Elena Blundo, Paulo E. Faria Junior, Alessandro Surrente, Giorgio Pettinari, Mikhail A. Prosnikov, Katarzyna Olkowska-Pucko, Klaus Zollner, Tomasz Woźniak, Andrey Chaves, Tomasz Kazimierczuk, Marco Felici, Adam Babiński, Maciej R. Molas, Peter C. M. Christianen, Jaroslav Fabian, and Antonio Polimeni

Author(s): Elena Blundo, Paulo E. Faria Junior, Alessandro Surrente, Giorgio Pettinari, Mikhail A. Prosnikov, Katarzyna Olkowska-Pucko, Klaus Zollner, Tomasz Woźniak, Andrey Chaves, Tomasz Kazimierczuk, Marco Felici, Adam Babiński, Maciej R. Molas, Peter C. M. Christianen, Jaroslav Fabian, and Antonio Polimeni

Mechanical deformations and ensuing strain are routinely exploited to tune the band gap energy and to enhance the functionalities of two-dimensional crystals. In this Letter, we show that strain leads also to a strong modification of the exciton magnetic moment in WS2 monolayers. Zeeman-splitting me…


[Phys. Rev. Lett. 129, 067402] Published Thu Aug 04, 2022

15 Aug 07:38

Six-Body and Eight-Body Exciton States in Monolayer ${\mathrm{WSe}}_{2}$

by Dinh Van Tuan, Su-Fei Shi, Xiaodong Xu, Scott A. Crooker, and Hanan Dery

Author(s): Dinh Van Tuan, Su-Fei Shi, Xiaodong Xu, Scott A. Crooker, and Hanan Dery

In the archetypal monolayer semiconductor WSe2, the distinct ordering of spin-polarized valleys (low-energy pockets) in the conduction band allows for studies of not only simple neutral excitons and charged excitons (i.e., trions), but also more complex many-body states that are predicted at higher …


[Phys. Rev. Lett. 129, 076801] Published Tue Aug 09, 2022

22 Jul 12:05

[ASAP] One-Step Growth of Bilayer 2H–1T′ MoTe2 van der Waals Heterostructures with Interlayer-Coupled Resonant Phonon Vibration

by Zenglong Guo, Lei Wang, Mengjiao Han, Erding Zhao, Liang Zhu, Weiteng Guo, Junyang Tan, Bilu Liu, Xing-Qiu Chen, and Junhao Lin

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ACS Nano
DOI: 10.1021/acsnano.2c04664
20 Jul 10:02

[ASAP] Controlling Spin–Orbit Coupling to Tailor Type-II Dirac Bands

by Nguyen Huu Lam, Phuong Lien Nguyen, Byoung Ki Choi, Trinh Thi Ly, Ganbat Duvjir, Tae Gyu Rhee, Yong Jin Jo, Tae Heon Kim, Chris Jozwiak, Aaron Bostwick, Eli Rotenberg, Younghun Hwang, Young Jun Chang, Jaekwang Lee, and Jungdae Kim

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ACS Nano
DOI: 10.1021/acsnano.2c04301
20 Jul 10:01

[ASAP] Large-Scale 1T′-Phase Tungsten Disulfide Atomic Layers Grown by Gas-Source Chemical Vapor Deposition

by Mitsuhiro Okada, Jiang Pu, Yung-Chang Lin, Takahiko Endo, Naoya Okada, Wen-Hsin Chang, Anh Khoa Augustin Lu7, Takeshi Nakanishi, Tetsuo Shimizu, Toshitaka Kubo, Yasumitsu Miyata, Kazu Suenaga8, Taishi Takenobu, Takatoshi Yamada, and Toshifumi Irisawa

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ACS Nano
DOI: 10.1021/acsnano.2c05699
05 Jul 10:04

[ASAP] Synthesis of Group VIII Magnetic Transition-Metal-Doped Monolayer MoSe2

by Dingyi Shen, Bei Zhao&, Zucheng Zhang, Hongmei Zhang, Xiangdong Yang, Ziwei Huang, Bailing Li, Rong Song, Yejun Jin, Ruixia Wu, Bo Li, Jia Li, and Xidong Duan

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ACS Nano
DOI: 10.1021/acsnano.2c02214
17 Jun 10:23

[ASAP] Observation of Magnetism-Induced Topological Edge State in Antiferromagnetic Topological Insulator MnBi4Te7

by Hao-Ke Xu, Mingqiang Gu, Fucong Fei, Yi-Sheng Gu, Dang Liu, Qiao-Yan Yu, Sha-Sha Xue, Xu-Hui Ning, Bo Chen, Hangkai Xie, Zhen Zhu, Dandan Guan, Shiyong Wang, Yaoyi Li, Canhua Liu, Qihang Liu, Fengqi Song, Hao Zheng, and Jinfeng Jia

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ACS Nano
DOI: 10.1021/acsnano.2c03622
17 Jun 10:23

[ASAP] Emergent and Tunable Topological Surface States in Complementary Sb/Bi2Te3 and Bi2Te3/Sb Thin-Film Heterostructures

by Yao Li, John W. Bowers, Joseph A. Hlevyack, Meng-Kai Lin, and Tai-Chang Chiang

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ACS Nano
DOI: 10.1021/acsnano.2c04639
17 Jun 10:21

Anomalous Contribution to the Nematic Electronic States from the Structural Transition in FeSe Revealed by Time- and Angle-Resolved Photoemission Spectroscopy

by Yuanyuan Yang, Qisi Wang, Shaofeng Duan, Hongliang Wo, Chaozhi Huang, Shichong Wang, Lingxiao Gu, Dao Xiang, Dong Qian, Jun Zhao, and Wentao Zhang

Author(s): Yuanyuan Yang, Qisi Wang, Shaofeng Duan, Hongliang Wo, Chaozhi Huang, Shichong Wang, Lingxiao Gu, Dao Xiang, Dong Qian, Jun Zhao, and Wentao Zhang

High-resolution time- and angle-resolved photoemission measurements were made on FeSe superconductors. With ultrafast photoexcitation, two critical excitation fluences that correspond to two ultrafast electronic phase transitions were found only in the dyz-orbit-derived band near the Brillouin-zone …


[Phys. Rev. Lett. 128, 246401] Published Mon Jun 13, 2022

10 Jun 12:15

[ASAP] Electrically Tunable Localized versus Delocalized Intralayer Moiré Excitons and Trions in a Twisted MoS2 Bilayer

by Medha Dandu, Garima Gupta, Pushkar Dasika, Kenji Watanabe, Takashi Taniguchi, and Kausik Majumdar

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ACS Nano
DOI: 10.1021/acsnano.2c00145
30 May 10:32

Chiral Excitonics in Monolayer Semiconductors on Patterned Dielectrics

by Xu-Chen Yang, Hongyi Yu, and Wang Yao

Author(s): Xu-Chen Yang, Hongyi Yu, and Wang Yao

Nano-optical excitation can inject exciton flow with left-right directionality controlled by circular polarization and angular directionality controlled by location of the excitation.


[Phys. Rev. Lett. 128, 217402] Published Mon May 23, 2022

05 May 09:29

[ASAP] Highly Tunable Carrier Tunneling in Vertical Graphene–WS2–Graphene van der Waals Heterostructures

by Zongqi Bai, Yang Xiao, Qing Luo, Miaomiao Li, Gang Peng, Zhihong Zhu, Fang Luo, Mengjian Zhu, Shiqiao Qin, and Kostya Novoselov

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ACS Nano
DOI: 10.1021/acsnano.2c00536
02 May 07:31

Is There a Polaron Signature in Angle-Resolved Photoemission of ${\mathrm{CsPbBr}}_{3}$?

by Maryam Sajedi, Maxim Krivenkov, Dmitry Marchenko, Jaime Sánchez-Barriga, Anoop K. Chandran, Andrei Varykhalov, Emile D. L. Rienks, Irene Aguilera, Stefan Blügel, and Oliver Rader

Author(s): Maryam Sajedi, Maxim Krivenkov, Dmitry Marchenko, Jaime Sánchez-Barriga, Anoop K. Chandran, Andrei Varykhalov, Emile D. L. Rienks, Irene Aguilera, Stefan Blügel, and Oliver Rader

The formation of large polarons has been proposed as reason for the high defect tolerance, low mobility, low charge carrier trapping, and low nonradiative recombination rates of lead halide perovskites. Recently, direct evidence for large-polaron formation has been reported from a 50% effective mass…


[Phys. Rev. Lett. 128, 176405] Published Fri Apr 29, 2022

26 Apr 13:55

[ASAP] Direct Spectroscopic Evidence of Magnetic Proximity Effect in MoS2 Monolayer on Graphene/Co

by Vladimir Voroshnin, Artem V. Tarasov, Kirill A. Bokai, Alla Chikina, Boris V. Senkovskiy, Niels Ehlen, Dmitry Yu. Usachov, Alexander Grüneis, Maxim Krivenkov, Jaime Sánchez-Barriga, and Alexander Fedorov

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ACS Nano
DOI: 10.1021/acsnano.1c10391
26 Apr 13:54

[ASAP] Electronic Band Tuning and Multivalley Raman Scattering in Monolayer Transition Metal Dichalcogenides at High Pressures

by Luiz G. Pimenta Martins, Bruno R. Carvalho, Connor A. Occhialini, Natália P. Neme, Ji-Hoon Park, Qian Song, Pedro Venezuela, Mário S. C. Mazzoni, Matheus J. S. Matos, Jing Kong, and Riccardo Comin

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ACS Nano
DOI: 10.1021/acsnano.2c01065
19 Apr 08:05

Anomalies at the Dirac Point in Graphene and Its Hole-Doped Compositions

by Arindam Pramanik, Sangeeta Thakur, Bahadur Singh, Philip Willke, Martin Wenderoth, Hans Hofsäss, Giovanni Di Santo, Luca Petaccia, and Kalobaran Maiti

Author(s): Arindam Pramanik, Sangeeta Thakur, Bahadur Singh, Philip Willke, Martin Wenderoth, Hans Hofsäss, Giovanni Di Santo, Luca Petaccia, and Kalobaran Maiti

We study the properties of the Dirac states in SiC-graphene and its hole-doped compositions employing angle-resolved photoemission spectroscopy and density functional theory. The symmetry-selective measurements for the Dirac bands reveal their linearly dispersive behavior across the Dirac point whic…


[Phys. Rev. Lett. 128, 166401] Published Mon Apr 18, 2022

05 Apr 13:32

[ASAP] Mapping 1D Confined Electromagnetic Edge States in 2D Monolayer Semiconducting MoS2 Using 4D-STEM

by Yi Wen, Shiang Fang, Matthew Coupin, Yang Lu, Colin Ophus, Efthimios Kaxiras, and Jamie H. Warner

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ACS Nano
DOI: 10.1021/acsnano.2c01170
05 Apr 13:27

High-Order Harmonic Generation and Its Unconventional Scaling Law in the Mott-Insulating ${\mathrm{Ca}}_{2}{\mathrm{RuO}}_{4}$

by K. Uchida, G. Mattoni, S. Yonezawa, F. Nakamura, Y. Maeno, and K. Tanaka

Author(s): K. Uchida, G. Mattoni, S. Yonezawa, F. Nakamura, Y. Maeno, and K. Tanaka

Competition and cooperation among orders is at the heart of many-body physics in strongly correlated materials and leads to their rich physical properties. It is crucial to investigate what impact many-body physics has on extreme nonlinear optical phenomena, with the possibility of controlling mater…


[Phys. Rev. Lett. 128, 127401] Published Wed Mar 23, 2022

15 Mar 08:27

Imaging the Spatial Distribution of Electronic States in Graphene Using Electron Energy-Loss Spectroscopy: Prospect of Orbital Mapping

by M. Bugnet, M. Ederer, V. K. Lazarov, L. Li, Q. M. Ramasse, S. Löffler, and D. M. Kepaptsoglou

Author(s): M. Bugnet, M. Ederer, V. K. Lazarov, L. Li, Q. M. Ramasse, S. Löffler, and D. M. Kepaptsoglou

The spatial distributions of antibonding π* and σ* states in epitaxial graphene multilayers are mapped using electron energy-loss spectroscopy in a scanning transmission electron microscope. Inelastic channeling simulations validate the interpretation of the spatially resolved signals in terms of el…


[Phys. Rev. Lett. 128, 116401] Published Mon Mar 14, 2022

07 Mar 08:33

[ASAP] Two-Dimensional Superconductivity of Ca-Intercalated Graphene on SiC: Vital Role of the Interface between Monolayer Graphene and the Substrate

by Haruko Toyama, Ryota Akiyama, Satoru Ichinokura, Mizuki Hashizume, Takushi Iimori, Yukihiro Endo, Rei Hobara, Tomohiro Matsui, Kentaro Horii, Shunsuke Sato, Toru Hirahara, Fumio Komori, and Shuji Hasegawa

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ACS Nano
DOI: 10.1021/acsnano.1c11161
07 Mar 08:29

[ASAP] Quantitatively Deciphering Electronic Properties of Defects at Atomically Thin Transition-Metal Dichalcogenides

by Si-Si Wu, Teng-Xiang Huang, Xiaolan Xu, Yi-Fan Bao, Xin-Di Pei, Xu Yao, Mao-Feng Cao, Kai-Qiang Lin, Xiang Wang, Dongdong Wang, and Bin Ren

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ACS Nano
DOI: 10.1021/acsnano.2c00096
07 Mar 07:32

Flat-Band-Induced Anomalous Anisotropic Charge Transport and Orbital Magnetism in Kagome Metal CoSn

by Hao Huang, Lixuan Zheng, Zhiyong Lin, Xu Guo, Sheng Wang, Shuai Zhang, Chi Zhang, Zhe Sun, Zhengfei Wang, Hongming Weng, Lin Li, Tao Wu, Xianhui Chen, and Changgan Zeng

Author(s): Hao Huang, Lixuan Zheng, Zhiyong Lin, Xu Guo, Sheng Wang, Shuai Zhang, Chi Zhang, Zhe Sun, Zhengfei Wang, Hongming Weng, Lin Li, Tao Wu, Xianhui Chen, and Changgan Zeng

For solids, the dispersionless flat band has long been recognized as an ideal platform for achieving intriguing quantum phases. However, experimental progress in revealing flat-band physics has so far been achieved mainly in artificially engineered systems represented as magic-angle twisted bilayer …


[Phys. Rev. Lett. 128, 096601] Published Mon Feb 28, 2022

21 Feb 09:04

[ASAP] CrxPt1–xTe2 (x ≤ 0.45): A Family of Air-Stable and Exfoliatable van der Waals Ferromagnets

by Warren L. B. Huey, Andrew M. Ochs, Archibald J. Williams, Yuxin Zhang, Simo Kraguljac, Ziling Deng, Curtis E. Moore, Wolfgang Windl, Chun Ning Lau, and Joshua E. Goldberger

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ACS Nano
DOI: 10.1021/acsnano.1c08681
07 Feb 09:35

Scattering between Minivalleys in Twisted Double Bilayer Graphene

by Petar Tomić, Peter Rickhaus, Aitor Garcia-Ruiz, Giulia Zheng, Elías Portolés, Vladimir Fal’ko, Kenji Watanabe, Takashi Taniguchi, Klaus Ensslin, Thomas Ihn, and Folkert K. de Vries

Author(s): Petar Tomić, Peter Rickhaus, Aitor Garcia-Ruiz, Giulia Zheng, Elías Portolés, Vladimir Fal’ko, Kenji Watanabe, Takashi Taniguchi, Klaus Ensslin, Thomas Ihn, and Folkert K. de Vries

Magnetotransport oscillations in twisted double bilayer graphene exhibit scattering between minivalleys that depends on both electron-phonon and electron-electron effects.


[Phys. Rev. Lett. 128, 057702] Published Fri Feb 04, 2022

01 Feb 12:57

Polarization-Modulated Angle-Resolved Photoemission Spectroscopy: Toward Circular Dichroism without Circular Photons and Bloch Wave-function Reconstruction

by Michael Schüler, Tommaso Pincelli, Shuo Dong, Thomas P. Devereaux, Martin Wolf, Laurenz Rettig, Ralph Ernstorfer, and Samuel Beaulieu

Author(s): Michael Schüler, Tommaso Pincelli, Shuo Dong, Thomas P. Devereaux, Martin Wolf, Laurenz Rettig, Ralph Ernstorfer, and Samuel Beaulieu

Complete characterization of certain quantum materials requires knowledge of the complex wave functions that describe electrons in the solid. A new measurement methodology provides deep insights into that information.


[Phys. Rev. X 12, 011019] Published Fri Jan 28, 2022

14 Jan 08:33

Valley-Polarized Quantum Anomalous Hall State in Moiré ${\mathrm{MoTe}}_{2}/{\mathrm{WSe}}_{2}$ Heterobilayers

by Ying-Ming Xie, Cheng-Ping Zhang, Jin-Xin Hu, Kin Fai Mak, and K. T. Law

Author(s): Ying-Ming Xie, Cheng-Ping Zhang, Jin-Xin Hu, Kin Fai Mak, and K. T. Law

Moiré heterobilayer transition metal dichalcogenides (TMDs) emerge as an ideal system for simulating the single-band Hubbard model and interesting correlated phases have been observed in these systems. Nevertheless, the moiré bands in heterobilayer TMDs were believed to be topologically trivial. Rec…


[Phys. Rev. Lett. 128, 026402] Published Tue Jan 11, 2022