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30 Nov 06:17

The compatibility of methylammonium and formamidinium in mixed cation perovskite: the optoelectronic and stability properties

by Xinlu Guo, Kwanho Ngai, Minchao Qin, Xinhu Lu, Jianbin Xu and Mingzhu Long
The methylammonium (MA) and formamidinium (FA) are the most commonly used organic cations in perovskite solar cells (PSCs), whereas the impact of size and polarity differences between these two on the photovoltaic performances has been rarely revealed. Herein, we systematically investigated the phase distribution, optoelectronic and stability properties of FA-MA mixed perovskites. To identify the phase homogeneity, depth-dependent grazing-incidence wide-angle x-ray scattering measurements were employed, which demonstrates that the mixed cation perovskite possesses a FA-rich phase on the film surface and the bottom is comprised of MA-rich phase. Additionally, upon long-time illumination, a new PL peak is appeared at 778 nm, representing the generation of MA-rich phase induced by ion migration. It is worth noting that the phase splitting and inhomogeneous phase distribution would not bring any obvious detrimental effects to the photovoltaic performances and stability properties. T...
30 Nov 06:15

Two compatible polymer donors contribute synergistically for ternary organic solar cells with 17.53% efficiency

Energy Environ. Sci., 2020, Advance Article
DOI: 10.1039/D0EE02516J, Paper
Qiaoshi An, Junwei Wang, Xiaoling Ma, Jinhua Gao, Zhenghao Hu, Bin Liu, Huiliang Sun, Xugang Guo, Xiaoli Zhang, Fujun Zhang
The optimized ternary organic solar cells achieve a PCE of 17.53% by synergizing two well-matched polymer donors.
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30 Nov 06:15

Polymeric room-temperature molten salt as a multifunctional additive toward highly efficient and stable inverted planar perovskite solar cells

Energy Environ. Sci., 2020, Advance Article
DOI: 10.1039/D0EE02043E, Paper
Shuangjie Wang, Bowen Yang, Jian Han, Ziwei He, Tongtong Li, Qi Cao, Jiabao Yang, Jiajia Suo, Xuanhua Li, Zhike Liu, Shengzhong (Frank) Liu, Chao Tang, Anders Hagfeldt
We for the first time report the application of a polymeric room-temperature molten salt in high efficiency and excellent stability inverted perovskite solar cells.
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30 Nov 06:15

Material perceptions and advances in molecular heteroacenes for organic solar cells

Energy Environ. Sci., 2020, 13,4738-4793
DOI: 10.1039/D0EE02461A, Review Article
Amaresh Mishra
This review showcases the development of heteroacene-based molecular materials and their role in high performance binary, ternary, tandem and semitransparent organic solar cells.
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30 Nov 06:14

Heat dissipation effects on the stability of planar perovskite solar cells

Energy Environ. Sci., 2020, Advance Article
DOI: 10.1039/D0EE02859B, Paper
Kyoungwon Choi, Junwoo Lee, Hyuntae Choi, Guan-Woo Kim, Hong Il Kim, Taiho Park
Highly stable planar perovskite solar cells without encapsulation were demonstrated by desirable heat dissipation and stable morphology of hole-transporting materials.
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30 Nov 06:13

Emerging Perovskite Quantum Dot Solar Cells:Feasible Approaches to Boost Performance

Energy Environ. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0EE02900A, Review Article
Jingxuan Chen, Donglin Jia, Erik M. J. Johansson, Anders Hagfeldt, Xiaoliang Zhang
Lead halide perovskite quantum dots (PQDs), also called perovskite nanocrystals, are considered as one of the most promising class of photovoltaic materials for solar cells due to their prominent optoelectronic...
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24 Nov 04:24

[ASAP] Design, Synthesis, and Photocatalytic Application of Moisture-Stable Hybrid Lead-Free Perovskite

by Guang-Ning Liu, Ruo-Yu Zhao, Bo Xu, Yiqiang Sun, Xiao-Ming Jiang, Xun Hu, and Cuncheng Li

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ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c16107
24 Nov 04:24

[ASAP] Enhancing the Efficiency and Stability of Triple-Cation Perovskite Solar Cells by Eliminating Excess PbI2 from the Perovskite/Hole Transport Layer Interface

by Zhelu Hu, Qingzhi An, Hengyang Xiang, Lionel Aigouy, Baoquan Sun, Yana Vaynzof, and Zhuoying Chen

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ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c17258
22 Nov 06:56

Progress in Materials Development for Flexible Perovskite Solar Cells and Future Prospects

by Snehangshu Mishra, Subrata Ghosh, Trilok Singh
Progress in Materials Development for Flexible Perovskite Solar Cells and Future Prospects

Your flexible friend: Flexible perovskite solar cells have potential applications in portable electronics, wearable power sources, electronic textiles, and large‐scale industrial roofing, owing to its high efficiency, lightweight, flexibility, and suitability for roll‐to‐roll production. This Review summarizes the development of materials for flexible perovskite solar cells.


Abstract

The perovskite solar cells (PSCs) have emerged as an established technology during the last decade, with the record efficiency of such solar cells having increased from 3.8 % to 25.5 %. Recently, flexible perovskite solar cells (fPSCs) have received much attention from the academic and the industrial communities, owing to their potential for various niche applications, including portable electronics, wearable power sources, electronic textiles, and large‐scale industrial roofing. fPSCs are lightweight, bendable, and suitable for roll‐to‐roll industrial production and can be integrated easily over any surface. This Review discusses the recent development of materials for fPSCs based on various flexible substrates, including plastic, metal, and other flexible substrates, as well as fiber‐shaped perovskite solar cells, with a focus on the device structure, material selection for each layer, mechanical flexibility and the environmental stability of the fPSC devices. Finally, future applications and the outlook for fPSCs are also discussed.

22 Nov 06:56

[ASAP] Printable Free-Standing Hybrid Graphene/Dry-Spun Carbon Nanotube Films as Multifunctional Electrodes for Highly Stable Perovskite Solar Cells

by Mengdi Tian, Chae Young Woo, Jin Woo Choi, Ji-Youn Seo, Jong-Man Kim, Soo Hyung Kim, Myungkwan Song, and Hyung Woo Lee

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ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c17141
21 Nov 09:43

[ASAP] Unusual Surface Ligand Doping-Induced p-Type Quantum Dot Solids and Their Application in Solar Cells

by Lingju Meng, Qiwei Xu, Ujwal K. Thakur, Lu Gong, Hongbo Zeng, Karthik Shankar, and Xihua Wang

TOC Graphic

ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c15576
19 Nov 07:19

Progress in Materials Development for Flexible Perovskite Solar Cells and Future Prospects

by Snehangshu Mishra, Subrata Ghosh, Trilok Singh
Progress in Materials Development for Flexible Perovskite Solar Cells and Future Prospects

Your flexible friend: Flexible perovskite solar cells have potential applications in portable electronics, wearable power sources, electronic textiles, and large‐scale industrial roofing, owing to its high efficiency, lightweight, flexibility, and suitability for roll‐to‐roll production. This Review summarizes the development of materials for flexible perovskite solar cells.


Abstract

The perovskite solar cells (PSCs) have emerged as an established technology during the last decade, with the record efficiency of such solar cells having increased from 3.8 % to 25.5 %. Recently, flexible perovskite solar cells (fPSCs) have received much attention from the academic and the industrial communities, owing to their potential for various niche applications, including portable electronics, wearable power sources, electronic textiles, and large‐scale industrial roofing. fPSCs are lightweight, bendable, and suitable for roll‐to‐roll industrial production and can be integrated easily over any surface. This Review discusses the recent development of materials for fPSCs based on various flexible substrates, including plastic, metal, and other flexible substrates, as well as fiber‐shaped perovskite solar cells, with a focus on the device structure, material selection for each layer, mechanical flexibility and the environmental stability of the fPSC devices. Finally, future applications and the outlook for fPSCs are also discussed.

18 Nov 09:04

[ASAP] Nanoparticle Wetting Agent for Gas Stream-Assisted Blade-Coated Inverted Perovskite Solar Cells and Modules

by Johannes Küffner, Tina Wahl, Moritz Schultes, Jonas Hanisch, Julia Zillner, Erik Ahlswede, and Michael Powalla

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ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c15428
18 Nov 09:04

[ASAP] MXene-Modulated Electrode/SnO2 Interface Boosting Charge Transport in Perovskite Solar Cells

by Yunfan Wang, Pan Xiang, Aobo Ren, Huagui Lai, Zhuoqiong Zhang, Zhipeng Xuan, Zhenxi Wan, Jingquan Zhang, Xia Hao, Lili Wu, Masakazu Sugiyama, Udo Schwingenschlögl, Cai Liu, Zeguo Tang, Jiang Wu, Zhiming Wang, and Dewei Zhao

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ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c17338
17 Nov 08:11

[ASAP] Sodium Dodecylbenzene Sulfonate Interface Modification of Methylammonium Lead Iodide for Surface Passivation of Perovskite Solar Cells

by Yuqin Zou, Renjun Guo, Ali Buyruk, Wei Chen, Tianxiao Xiao, Shanshan Yin, Xinyu Jiang, Lucas P. Kreuzer, Cheng Mu, Tayebeh Ameri, Matthias Schwartzkopf, Stephan V. Roth, and Peter Müller-Buschbaum

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ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c14732
08 Nov 13:35

A Dendrite‐Structured RbX (X=Br, I) Interlayer for CsPbI2Br Perovskite Solar Cells with Over 15 % Stabilized Efficiency

by Jingjing He, Bing Ge, Yu Hou, Shuang Yang, Hua Gui Yang
A Dendrite‐Structured RbX (X=Br, I) Interlayer for CsPbI2Br Perovskite Solar Cells with Over 15 % Stabilized Efficiency

“Interface engineering is an important strategy for perovskite solar cells…” This and more about the story behind the research that inspired the Cover image is presented in the Cover Profile. Read the full text of the corresponding research at 10.1002/cssc.202001629. View the Front Cover here: 10.1002/cssc.202002047.


Abstract

Invited for this month′s cover is the group of Shuang Yang at the East China University of Science and Technology. The image shows a dendrite‐structured interlayer for CsPbI2Br perovskite solar cells. The Full Paper itself is available at 10.1002/cssc.202001629.

08 Nov 13:35

Toward ideal hole transport materials: a review on recent progress in dopant-free hole transport materials for fabricating efficient and stable perovskite solar cells

Energy Environ. Sci., 2020, 13,4057-4086
DOI: 10.1039/D0EE02337J, Review Article
Xinxing Yin, Zhaoning Song, Zaifang Li, Weihua Tang
A review on the fundamental understanding and rational design of ideal, dopant-free HTMs for fabricating efficient and stable perovskite solar cells.
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08 Nov 13:35

[ASAP] Incorporation of Lithium Fluoride Restraining Thermal Degradation and Photodegradation of Organometal Halide Perovskite Solar Cells

by Alan Jiwan Yun, Jinhyun Kim, Bumjin Gil, Hyungsub Woo, Kimin Park, Jaemin Cho, and Byungwoo Park

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ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c14218
08 Nov 13:35

[ASAP] Luminescent, Wide-Band Gap Solar Cells with a Photovoltage up to 1.75 V through a Heterostructured Light-Absorbing Layer

by Dingjian Zhou, Jincheng Huang, Huibo Yan, Jianfeng Zhang, Lei Lu, Ping Xu, and Guijun Li

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ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c16032
08 Nov 13:35

[ASAP] Novel Quasi-2D Perovskites for Stable and Efficient Perovskite Solar Cells

by Tao Zhu, Yongrui Yang, Kai Gu, Chunming Liu, Jie Zheng, and Xiong Gong

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ACS Applied Materials & Interfaces
DOI: 10.1021/acsami.0c16514