Shared posts

01 Jul 12:50

Creating Ferroelectricity in Monoclinic $({\mathrm{HfO}}_{2}{)}_{1}/({\mathrm{CeO}}_{2}{)}_{1}$ Superlattices

by Hong Jian Zhao, Yuhao Fu, Longju Yu, Yanchao Wang, Yurong Yang, Laurent Bellaiche, and Yanming Ma

Author(s): Hong Jian Zhao, Yuhao Fu, Longju Yu, Yanchao Wang, Yurong Yang, Laurent Bellaiche, and Yanming Ma

Ferroelectricity in CMOS-compatible hafnia (HfO2) is crucial for the fabrication of high-integration nonvolatile memory devices. However, the capture of ferroelectricity in HfO2 requires the stabilization of thermodynamically metastable orthorhombic or rhombohedral phases, which entails the introduc…


[Phys. Rev. Lett. 132, 256801] Published Mon Jun 17, 2024

01 Jul 12:48

Deciphering in-situ surface reconstruction in two-dimensional CdPS3 nanosheets for efficient biomass hydrogenation

by Marshet Getaye Sendeku

Nature Communications, Published online: 18 June 2024; doi:10.1038/s41467-024-49510-8

Targeting the electrosynthesis of valuable chemicals from biomass-based feedstocks requires understanding the phenomena at the interface and electrode surface. Here, the authors demonstrate electrolyte-driven surface reconstruction on layered CdPS3 nanosheets for the efficient hydrogenation of 5-hydroxymethylfurfural.
01 Jul 12:47

Author Correction: Waveguide-integrated twisted bilayer graphene photodetectors

by Qinci Wu

Nature Communications, Published online: 21 June 2024; doi:10.1038/s41467-024-49561-x

Author Correction: Waveguide-integrated twisted bilayer graphene photodetectors
01 Jul 12:42

Intrinsic-strain-induced ferroelectric order and ultrafine nanodomains in SrTiO3

by Peixi ZhangQiang LiZhiguo LiXiaoming ShiHaoyu WangChuanrui HuoLihui ZhouXiaojun KuangKun LinYili CaoJinxia DengChengyi YuXin ChenJun MiaoXianran XingaBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Solid State Chemistry, University of Science and Technology Beijing, Beijing 100083, ChinabDepartment of Physics, University of Science and Technology Beijing, Beijing 100083, ChinacBeijing Advanced Innovation Center for Materials Genome Engineering, Department of Physical Chemistry, University of Science and Technology Beijing, Beijing 100083, ChinadKey Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Feringa Nobel Prize Scientist Joint Research Center, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, ChinaeGuangxi Key Laboratory of Electrochemical and Magnetochemical Functional Materials, College of Chemistry and Bioengineering, Guilin University of Technology, Guilin 541006, China
Proceedings of the National Academy of Sciences, Volume 121, Issue 25, June 2024.
01 Jul 12:35

Charge-depletion-enhanced WSe2 quantum emitters on gold nanogap arrays with near-unity quantum efficiency

by Hongbing Cai

Nature Photonics, Published online: 17 June 2024; doi:10.1038/s41566-024-01460-9

Non-radiative decay in two-dimensional WSe2 quantum emitters is electrically suppressed through charge depletion using dual gate configurations. The single-photon emitter transition quantum efficiency after gating is increased to 76.4 ± 14.6% on average.
01 Jul 12:35

Transport and localization of indirect excitons in a van der Waals heterostructure

by L. H. Fowler-Gerace

Nature Photonics, Published online: 18 June 2024; doi:10.1038/s41566-024-01435-w

Spatial distribution of the photoluminescence of interlayer excitons in van der Waals heterostructures comprising MoSe2 and WSe2 monolayers and encapsulated in rather thick hexagonal boron nitride is investigated, revealing interlayer exciton long-range transport with 1/e decay distances reaching and exceeding 100 μm.
01 Jul 12:29

Tunable superconductivity in electron- and hole-doped Bernal bilayer graphene

by Chushan Li

Nature, Published online: 19 June 2024; doi:10.1038/s41586-024-07584-w

Tunable superconductivity and a series of flavour-symmetry-breaking phases are observed in electron- and hole-doped Bernal bilayer graphene.
01 Jul 12:29

Control of proton transport and hydrogenation in double-gated graphene

by J. Tong

Nature, Published online: 19 June 2024; doi:10.1038/s41586-024-07435-8

Independent control of the electric field and charge-carrier density in double-gated graphene allows the decoupling of proton transport and lattice hydrogenation, enabling both accelerated proton transport and proton-based logic operations.
17 Jun 01:41

Correlated Charge Density Wave Insulators in Chirally Twisted Triple Bilayer Graphene

by Wenxuan Wang, Gengdong Zhou, Wenlu Lin, Zuo Feng, Yijie Wang, Miao Liang, Zaizhe Zhang, Min Wu, Le Liu, Kenji Watanabe, Takashi Taniguchi, Wei Yang, Guangyu Zhang, Kaihui Liu, Jinhua Gao, Yang Liu, X. C. Xie, Zhida Song, and Xiaobo Lu

Author(s): Wenxuan Wang, Gengdong Zhou, Wenlu Lin, Zuo Feng, Yijie Wang, Miao Liang, Zaizhe Zhang, Min Wu, Le Liu, Kenji Watanabe, Takashi Taniguchi, Wei Yang, Guangyu Zhang, Kaihui Liu, Jinhua Gao, Yang Liu, X. C. Xie, Zhida Song, and Xiaobo Lu

A high-quality device made from a new moiré structure formed by three pieces of helically stacked Bernal bilayer graphene functions as a highly tunable flat-band system.


[Phys. Rev. Lett. 132, 246501] Published Mon Jun 10, 2024

17 Jun 01:40

Double and Quadruple Flat Bands Tuned by Alternative Magnetic Fluxes in Twisted Bilayer Graphene

by Congcong Le, Qiang Zhang, Fan Cui, Xianxin Wu, and Ching-Kai Chiu

Author(s): Congcong Le, Qiang Zhang, Fan Cui, Xianxin Wu, and Ching-Kai Chiu

Twisted bilayer graphene (TBG) can host the moiré energy flat bands with twofold degeneracy serving as a fruitful playground for strong correlations and topological phases. However, the number of degeneracy is not limited to two. Introducing a spatially alternative magnetic field, we report that the…


[Phys. Rev. Lett. 132, 246401] Published Thu Jun 13, 2024

17 Jun 01:40

Exciton-Enhanced Spontaneous Parametric Down-Conversion in Two-Dimensional Crystals

by Fengyuan Xuan, MingRui Lai, Yaze Wu, and Su Ying Quek

Author(s): Fengyuan Xuan, MingRui Lai, Yaze Wu, and Su Ying Quek

We show that excitonic resonances and interexciton transitions can enhance the probability of spontaneous parametric down-conversion, a second-order optical response that generates entangled photon pairs. We benchmark our ab initio many-body calculations using experimental polar plots of second harm…


[Phys. Rev. Lett. 132, 246902] Published Fri Jun 14, 2024

17 Jun 01:40

Signatures of Kitaev Interactions in the van der Waals Ferromagnet ${\mathrm{VI}}_{3}$

by Yiqing Gu, Yimeng Gu, Feiyang Liu, Seiko Ohira-Kawamura, Naoki Murai, and Jun Zhao

Author(s): Yiqing Gu, Yimeng Gu, Feiyang Liu, Seiko Ohira-Kawamura, Naoki Murai, and Jun Zhao

Inelastic neutron scattering measurements on VI3, a two-dimensional ferromagnetic Mott insulator, reveal distinct anisotropic magnetic excitations that are described by a model with large bond-dependent Kitaev interactions.


[Phys. Rev. Lett. 132, 246702] Published Fri Jun 14, 2024

17 Jun 01:40

Symmetry-Broken Perturbation Theory to Large Orders in Antiferromagnetic Phases

by Renaud Garioud, Fedor Šimkovic, IV, Riccardo Rossi, Gabriele Spada, Thomas Schäfer, Félix Werner, and Michel Ferrero

Author(s): Renaud Garioud, Fedor Šimkovic, IV, Riccardo Rossi, Gabriele Spada, Thomas Schäfer, Félix Werner, and Michel Ferrero

We introduce a spin-symmetry-broken extension of the connected determinant algorithm [Riccardo Rossi, Determinant diagrammatic Monte Carlo algorithm in the thermodynamic limit, Phys. Rev. Lett. 119, 045701 (2017).]. The resulting systematic perturbative expansions around an antiferromagnetic state a…


[Phys. Rev. Lett. 132, 246505] Published Fri Jun 14, 2024

17 Jun 01:39

Local Noise Spectroscopy of Wigner Crystals in Two-Dimensional Materials

by Pavel E. Dolgirev, Ilya Esterlis, Alexander A. Zibrov, Mikhail D. Lukin, Thierry Giamarchi, and Eugene Demler

Author(s): Pavel E. Dolgirev, Ilya Esterlis, Alexander A. Zibrov, Mikhail D. Lukin, Thierry Giamarchi, and Eugene Demler

We propose local electromagnetic noise spectroscopy as a versatile and noninvasive tool to study Wigner crystal phases of strongly interacting two-dimensional electronic systems. In-plane imaging of the local noise is predicted to enable single-site resolution of the electron crystal when the sample…


[Phys. Rev. Lett. 132, 246504] Published Fri Jun 14, 2024

17 Jun 01:39

Directional Localization from a Magnetic Field in Moiré Systems

by Nisarga Paul, Philip J. D. Crowley, and Liang Fu

Author(s): Nisarga Paul, Philip J. D. Crowley, and Liang Fu

Moiré materials provide a highly tunable platform in which novel electronic phenomena can emerge. We study strained moiré materials in a uniform magnetic field and predict highly anisotropic electrical conductivity that switches easy axis as magnetic field or strain is varied. The dramatic anisotrop…


[Phys. Rev. Lett. 132, 246402] Published Fri Jun 14, 2024

17 Jun 01:36

Combining ultrahigh index with exceptional nonlinearity in resonant transition metal dichalcogenide nanodisks

by George Zograf

Nature Photonics, Published online: 13 June 2024; doi:10.1038/s41566-024-01444-9

Using the 3R phase of molybdenum disulfide nanodisks with various radii, more than 100-fold enhancement of second-harmonic generation can be obtained in a single resonant nanodisk compared with an unpatterned flake of the same thickness.
17 Jun 01:35

Strong chiroptical nonlinearity in coherently stacked boron nitride nanotubes

by Chaojie Ma

Nature Nanotechnology, Published online: 06 June 2024; doi:10.1038/s41565-024-01685-3

Multiwalled boron nitride nanotubes, featuring coherently stacked structures with monochirality, homo-handedness and unipolarity among the component tubes, show a large nonlinear chiroptical response.
17 Jun 01:29

Ultra-high spin emission from antiferromagnetic FeRh

by Dominik Hamara

Nature Communications, Published online: 11 June 2024; doi:10.1038/s41467-024-48795-z

The authors measure picosecond spin pumping in FeRh as a function of temperature by optical pump-THz emission spectroscopy. In the antiferromagnetic phase of FeRh enhanced spin pumping above the value measured in the ferromagnetic phase is observed.
17 Jun 01:28

Electrical noise spectroscopy of magnons in a quantum Hall ferromagnet

by Ravi Kumar

Nature Communications, Published online: 12 June 2024; doi:10.1038/s41467-024-49446-z

Quantum Hall ferromagnets can host magnons, collective spin-wave excitations, which have possible uses in spin-wave based information processing. Detecting these excitations electrically can be challenging. Here, Kumar, Srivastav, Roy, Park and coauthors demonstrate a noise-based approach to detecting magnons.
17 Jun 01:21

A two-site Kitaev chain in a two-dimensional electron gas

by Sebastiaan L. D. ten Haaf

Nature, Published online: 12 June 2024; doi:10.1038/s41586-024-07434-9

We have implemented a two-site Kitaev chain in a two-dimensional electron gas by coupling quantum dots through Andreev bound states in a superconductor–semiconductor hybrid region.
11 Jun 02:33

Epitaxial growth of quantum dots on van der Waals surfaces

by Kaiyao Xin

Nature Synthesis, Published online: 04 June 2024; doi:10.1038/s44160-024-00562-0

A van der Waals epitaxial strategy is reported for growing intrinsic quantum dots (QDs) by modulating interfacial couplings on van der Waals surfaces. This method overcomes lattice mismatch constraints and produces versatile III–V and IV–VI QDs with controllable morphologies, broadening near-infrared photoresponse in InSb QDs/MoS2 by efficient interlayer charge transfer.
11 Jun 02:33

Local and Nonlocal Electronic Correlations at the Metal-Insulator Transition in the Two-Dimensional Hubbard Model

by Maria Chatzieleftheriou, Silke Biermann, and Evgeny A. Stepanov

Author(s): Maria Chatzieleftheriou, Silke Biermann, and Evgeny A. Stepanov

D-TRILEX calculations unveil details of the crossover region in Mott transitions between the weakly and strongly correlated regimes for a half-filled 2D Hubbard model.


[Phys. Rev. Lett. 132, 236504] Published Wed Jun 05, 2024

11 Jun 02:30

All-optical polarization switching in ferroelectrics

by Vasily V. Temnov

Nature Photonics, Published online: 06 June 2024; doi:10.1038/s41566-024-01452-9

Ultrafast optical experiments using narrow-bandwidth tunable IR laser pulses enable nonvolatile all-optical switching of ferroelectric polarization in BaTiO3 in the epsilon-near-zero regime.
11 Jun 02:29

High-temperature superconductivity with zero resistance and strange-metal behaviour in La3Ni2O7−δ

by Yanan Zhang

Nature Physics, Published online: 06 June 2024; doi:10.1038/s41567-024-02515-y

Some features resembling superconductivity at high temperature have been seen under pressure in La3Ni2O7, but a transition to a zero-resistance state has not been observed. Now transport studies demonstrate this transition, along with strange metallicity.
11 Jun 02:28

MXenes with ordered triatomic-layer borate polyanion terminations

by Dongqi Li

Nature Materials, Published online: 07 June 2024; doi:10.1038/s41563-024-01911-2

MXenes with borate polyanion terminations are synthesized using a flux-assisted eutectic molten etching approach. These triatomic-layer terminations empower MXenes with considerably improved charge transport and charge storage capabilities.
11 Jun 02:20

Large-area, self-healing block copolymer membranes for energy conversion

by Christian C. M. Sproncken

Nature, Published online: 05 June 2024; doi:10.1038/s41586-024-07481-2

We introduce a self-assembly strategy that uses the interface of an aqueous two-phase system to template and stabilize molecularly thin biomimetic block copolymer bilayers of scalable area that can exceed 10 cm2 without defects.
11 Jun 02:18

Observation of 2D-magnesium-intercalated gallium nitride superlattices

by Jia Wang

Nature, Published online: 05 June 2024; doi:10.1038/s41586-024-07513-x

The spontaneous formation of magnesium-intercalated gallium nitride superlattices by the interstitial intercalation of two-dimensional magnesium results in considerable compressive strain perpendicular to the layers, leading to enhanced hole transport.
03 Jun 00:57

High-Temperature Anomalous Metal States in Iron-Based Interface Superconductors

by Yanan Li, Haiwen Liu, Haoran Ji, Chengcheng Ji, Shichao Qi, Xiaotong Jiao, Wenfeng Dong, Yi Sun, Wenhao Zhang, Zihan Cui, Minghu Pan, Nitin Samarth, Lili Wang, X. C. Xie, Qi-Kun Xue, Yi Liu, and Jian Wang

Author(s): Yanan Li, Haiwen Liu, Haoran Ji, Chengcheng Ji, Shichao Qi, Xiaotong Jiao, Wenfeng Dong, Yi Sun, Wenhao Zhang, Zihan Cui, Minghu Pan, Nitin Samarth, Lili Wang, X. C. Xie, Qi-Kun Xue, Yi Liu, and Jian Wang

The nature of the anomalous metal state has been a major puzzle in condensed matter physics for more than three decades. Here, we report systematic investigation and modulation of the anomalous metal states in high-temperature interface superconductor FeSe films on SrTiO3 substrate. Remarkably, unde…


[Phys. Rev. Lett. 132, 226003] Published Fri May 31, 2024

03 Jun 00:53

Photocatalytic toluene oxidation with nickel-mediated cascaded active units over Ni/Bi2WO6 monolayers

by Yingzhang Shi

Nature Communications, Published online: 31 May 2024; doi:10.1038/s41467-024-49005-6

By introducing Ni dopants into monolayer Bi2WO6, Bi/O frustrated Lewis pairs, unsaturated W atoms, and Ni active units are formed. The authors show that these units facilitate oxygen species transfer and enhance photocatalytic toluene oxidation.
03 Jun 00:53

A dual spin-controlled chiral two-/three-dimensional perovskite artificial leaf for efficient overall photoelectrochemical water splitting

by Hyungsoo Lee

Nature Communications, Published online: 01 June 2024; doi:10.1038/s41467-024-49216-x

Enhancing the efficiency of solar-driven water splitting is challenging but highly interesting. Here the authors report a dual spin-controlled 2D/3D perovskite photoelectrode that achieves 12.55% efficiency by utilizing the chiral-induced spin selectivity phenomenon.