Shared posts

11 Mar 02:41

[ASAP] Recent Progress of Amorphous Nanomaterials

by Jianxin Kang, Xiuyi Yang, Qi Hu, Zhi Cai, Li-Min Liu, and Lin Guo

TOC Graphic

Chemical Reviews
DOI: 10.1021/acs.chemrev.3c00229
24 Jul 04:06

[ASAP] Polymorphism and Ferroelectricity in Indium(III) Selenide

by Clement Kok Yong Tan, Wei Fu, and Kian Ping Loh

TOC Graphic

Chemical Reviews
DOI: 10.1021/acs.chemrev.3c00129
03 Jul 03:03

Synthesis of two-dimensional polyoxoniobate-based clusterphenes with in-plane electron delocalization

by Zhong Li

Nature Synthesis, Published online: 18 May 2023; doi:10.1038/s44160-023-00305-7

Polyoxoniobate (PONb) clusters are ideal candidates for synthesizing 2D clusterphenes but niobate reactivity is low. Now, 2D hexagonal PONb-clusterphenes have been prepared through a wet-chemical synthesis at ambient conditions, providing atomically precise models for examination of cluster electronic structures.
03 Jul 03:02

Synthesis of monolayer and persistent bilayer graphene fragments by using a radical-mediated coupling approach

by Tianyu Jiao

Nature Synthesis, Published online: 15 June 2023; doi:10.1038/s44160-023-00348-w

Atomically precise graphene fragments are synthesized by using a radical-mediated coupling approach. One open-shell doublet graphene fragment forms a persistent bilayer assembly with highly delocalized 32-centre-2-electron pancake bonding.
03 Jul 03:00

Electrically tunable moiré magnetism in twisted double bilayers of chromium triiodide

by Guanghui Cheng

Nature Electronics, Published online: 19 June 2023; doi:10.1038/s41928-023-00978-0

The magnetic state of twisted double bilayers of antiferromagnetic chromium triiodide can be controlled by electrical gating, twist angle and temperature.
03 Jul 02:55

Dirac revivals drive a resonance response in twisted bilayer graphene

by Erin Morissette

Nature Physics, Published online: 11 May 2023; doi:10.1038/s41567-023-02060-0

Phase transitions during which electrons recover their Dirac nature are shown to produce a spin resonance response that allows the characterization of spin and valley couplings in twisted bilayer graphene.
03 Jul 02:55

Evidence of non-collinear spin texture in magnetic moiré superlattices

by Hongchao Xie

Nature Physics, Published online: 18 May 2023; doi:10.1038/s41567-023-02061-z

A moiré potential may play a role in determining the magnetic properties of a two-dimensional homo or heterostructure. Now, non-collinear spin structures are observed in twisted double bilayer CrI3, providing a platform to engineer unusual magnetic textures.
03 Jul 02:54

Nanoscale electrostatic control in ultraclean van der Waals heterostructures by local anodic oxidation of graphite gates

by Liam A. Cohen

Nature Physics, Published online: 26 June 2023; doi:10.1038/s41567-023-02114-3

Precise control of electrons in two-dimensional materials has been limited by fabrication techniques for local gates that introduce disorder. Now, a technique allows patterning of sub-100 nm features and fabrication of very clean interfaces.
03 Jul 02:52

Electrical switching of ferro-rotational order in nanometre-thick 1T-TaS2 crystals

by Gan Liu

Nature Nanotechnology, Published online: 11 May 2023; doi:10.1038/s41565-023-01403-5

Domain wall formation and propagation using a small electric voltage are demonstrated in ferro-rotational 1T-TaS2, although the ferroic order does not couple with electromagnetic fields, providing an opportunity for the manipulation and application of ferro-rotational order.
03 Jul 02:52

Scalable CMOS back-end-of-line-compatible AlScN/two-dimensional channel ferroelectric field-effect transistors

by Kwan-Ho Kim

Nature Nanotechnology, Published online: 22 May 2023; doi:10.1038/s41565-023-01399-y

A large array of ferroelectric field-effect transistors with record memory windows, ON/OFF ratios and ON-current density is presented at ~80 nm channel length.
03 Jul 02:46

Layered materials as a platform for quantum technologies

by Alejandro R.-P. Montblanch

Nature Nanotechnology, Published online: 15 June 2023; doi:10.1038/s41565-023-01354-x

This Review highlights the role of transition metal dichalcogenides, hexagonal boron nitride and stacked heterostructures in applications in quantum communication, computation, sensing and single-photon detection.
03 Jul 02:46

Pressure tuning of minibands in MoS2/WSe2 heterostructures revealed by moiré phonons

by Luiz G. Pimenta Martins

Nature Nanotechnology, Published online: 15 June 2023; doi:10.1038/s41565-023-01413-3

Hydrostatic pressure is an underexplored tuning knob to study moiré systems. Here a MoS2/WSe2 heterostructure is compressed and the enhancement in the moiré potential strength is quantified via moiré-activated Raman modes.
03 Jul 02:45

Electro-thermal actuation in percolative ferroelectric polymer nanocomposites

by Yang Liu

Nature Materials, Published online: 25 May 2023; doi:10.1038/s41563-023-01564-7

Piezoelectric actuators play a critical role in precision positioning devices; however, materials with high actuation strain and mechanical energy density are rare. Here a composite of poly(vinylidene fluoride) and TiO2 demonstrates superior performance in these metrics, with the ferroelectric transition driven by Joule heating.
03 Jul 02:41

Exceptionally high charge mobility in phthalocyanine-based poly(benzimidazobenzophenanthroline)-ladder-type two-dimensional conjugated polymers

by Mingchao Wang

Nature Materials, Published online: 19 June 2023; doi:10.1038/s41563-023-01581-6

Linear π-conjugated polymers have attracted great attention as semiconductors for (opto)electronic devices, but charge transfer is only effective along polymer chains. Here poly(benzimidazobenzophenanthroline)-ladder-type two-dimensional conjugated polymers are presented with high charge carrier mobilities.
03 Jul 02:41

A twist for nanolight

by Siyuan Dai

Nature Materials, Published online: 22 June 2023; doi:10.1038/s41563-023-01586-1

Controlling the twist angles between three α-phase molybdenum trioxide single layers enables the programmable and reconfigurable canalization of phonon polaritons along multiple in-plane directions.
03 Jul 02:41

Spontaneous orbital polarization in the nematic phase of FeSe

by Connor A. Occhialini

Nature Materials, Published online: 22 June 2023; doi:10.1038/s41563-023-01585-2

FeSe does not exhibit magnetic order and lacks a nematic quantum critical point coinciding with optimal superconductivity, suggesting that an orbital mechanism drives nematicity, but direct evidence is lacking. Here, combining X-ray linear dichroism with in situ uniaxial stress, the role of spontaneous orbital polarization in nematic-phase FeSe is determined.
03 Jul 02:41

Intrinsic strong light-matter coupling with self-hybridized bound states in the continuum in van der Waals metasurfaces

by Thomas Weber

Nature Materials, Published online: 22 June 2023; doi:10.1038/s41563-023-01580-7

The authors demonstrate strong coupling in bound state in the continuum metasurfaces on nanostructured bulk WS2 and exhibiting sharp resonances with tailored linewidths and controllable light-matter coupling strength.
03 Jul 02:39

Operando electron microscopy investigation of polar domain dynamics in twisted van der Waals homobilayers

by Kahyun Ko

Nature Materials, Published online: 26 June 2023; doi:10.1038/s41563-023-01595-0

Polar domains have been observed in twist-stacked van der Waals layers, but their dynamics are unexplored. Here, using operando electron microscopy, it is found that polar domains in an antiferroelectric arrangement cannot transition to a ferroelectric state due to topological protection of the domain wall network.
03 Jul 02:38

Exciton-assisted electron tunnelling in van der Waals heterostructures

by Lujun Wang

Nature Materials, Published online: 26 June 2023; doi:10.1038/s41563-023-01556-7

The authors demonstrate exciton-assisted resonant electron tunnelling in van der Waals heterostructure tunnel junctions. Their study elucidates tunnelling mechanisms involving either indirect or direct excitons in the absence of charge injection and reveals excitonic light emission driven by inelastic electron tunnelling.
03 Jul 02:38

High-κ two-dimensional dielectric

by Taishi Takenobu

Nature Materials, Published online: 29 June 2023; doi:10.1038/s41563-023-01567-4

A two-dimensional atomically flat insulator with large dielectric constant and high breakdown field strength has been successfully grown. This material could serve as the dielectric and encapsulation layers for two-dimensional materials for studying their emergent physics, as well as for next-generation electronics.
03 Jul 02:37

Multistep, site-selective noncovalent synthesis of two-dimensional block supramolecular polymers

by Norihiko Sasaki

Nature Chemistry, Published online: 01 June 2023; doi:10.1038/s41557-023-01216-y

Supramolecular structures are typically formed by the one-step self-assembly of building blocks. Now, a greater level of control has been achieved using stepwise non-covalent reactions under kinetic control. Two-dimensional block supramolecular polymers with tailored compositions and sequences were synthesized, and a site selectivity that is reminiscent of regioselectivity in covalent synthesis was observed.
03 Jul 02:34

Signatures of Fractional Quantum Anomalous Hall States in Twisted MoTe2

by Jiaqi Cai

Nature, Published online: 14 June 2023; doi:10.1038/s41586-023-06289-w

Signatures of Fractional Quantum Anomalous Hall States in Twisted MoTe2
03 Jul 02:30

Magnetic-field-sensitive charge density waves in the superconductor UTe2

by Anuva Aishwarya

Nature, Published online: 28 June 2023; doi:10.1038/s41586-023-06005-8

A study using scanning tunnelling microscopy reveals a charge-density-wave state that is sensitive to magnetic fields and strongly intertwined with superconductivity in the heavy-fermion triplet superconductor UTe2.
03 Jul 02:26

Pair density wave state in a monolayer high-Tc iron-based superconductor

by Yanzhao Liu

Nature, Published online: 28 June 2023; doi:10.1038/s41586-023-06072-x

The primary pair density wave state has been discovered in a monolayer iron-based high-Tc superconductor, providing a platform to study the interplay between the correlated electronic states and unconventional Cooper pairing in high-Tc superconductors.
03 Jul 02:23

Detection of a pair density wave state in UTe2

by Qiangqiang Gu

Nature, Published online: 28 June 2023; doi:10.1038/s41586-023-05919-7

A spin-triplet pair density wave is discovered in the candidate topological superconductor UTe2 using superconductive scanning tunnelling microscopy tips.
04 May 12:25

Switchable moiré potentials in ferroelectric WTe2/WSe2 superlattices

by Kaifei Kang

Nature Nanotechnology, Published online: 27 April 2023; doi:10.1038/s41565-023-01376-5

Intrinsic ferroelectricity in bilayer WTe2 can be used for electrical switching of the centred-rectangular moiré potential in WTe2/WSe2 heterostructures.
04 May 12:24

Distinguishing atomic vibrations near point defects

by Xingxu Yan

Nature Materials, Published online: 03 May 2023; doi:10.1038/s41563-023-01538-9

Local vibrational modes at substitutional impurities in monolayer graphene are resolved with a sensitivity at the chemical bonding level, revealing the impacts of different chemical configurations and mass of impurity atoms on the defect-perturbed vibrational properties.
04 May 12:23

Lessons from hafnium dioxide-based ferroelectrics

by Beatriz Noheda

Nature Materials, Published online: 03 May 2023; doi:10.1038/s41563-023-01507-2

The discovery of ferroelectric switching in ultrathin layers of hafnium dioxide has aroused significant interest for low-power non-volatile memory technologies. This Perspective discusses how lessons learned from hafnium dioxide-based ferroelectrics can be applied to other applications, and other binary oxides.
04 May 12:18

Publisher Correction: 2D fin field-effect transistors integrated with epitaxial high-k gate oxide

by Congwei Tan

Nature, Published online: 03 May 2023; doi:10.1038/s41586-023-06093-6

Publisher Correction: 2D fin field-effect transistors integrated with epitaxial high-k gate oxide
04 May 12:17

Photo-induced high-temperature ferromagnetism in YTiO3

by A. S. Disa

Nature, Published online: 03 May 2023; doi:10.1038/s41586-023-05853-8

All-optical, mode-selective manipulation of the crystal lattice can be used to enhance and stabilize ferromagnetism in YTiO3 well above its equilibrium ordering temperature and for many nanoseconds, enabling dynamic engineering of practically useful non-equilibrium functionalities in fluctuating electronic systems.