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28 Feb 08:30

[ASAP] Fundament and Application of Graphdiyne in Electrochemical Energy

by Yuncheng Du†, Weidong Zhou*†, Jian Gao†, Xiangyu Pan†, and Yuliang Li*‡

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Accounts of Chemical Research
DOI: 10.1021/acs.accounts.9b00558
28 Feb 08:23

[ASAP] On-Surface Synthesis and Characterization of a Cycloarene: C108 Graphene Ring

by Qitang Fan†#, Daniel Martin-Jimenez‡#, Simon Werner†#, Daniel Ebeling*‡, Tabea Koehler†, Tobias Vollgraff†, Jo¨rg Sundermeyer*†, Wolfgang Hieringer§, Andre´ Schirmeisen‡, and J. Michael Gottfried*†

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b10151
28 Feb 08:23

[ASAP] Topological Defect-Induced Magnetism in a Nanographene

by Shantanu Mishra†, Doreen Beyer§, Reinhard Berger§, Junzhi Liu§, Oliver Gro¨ning†, Jose´ I. Urgel†, Klaus Mu¨llen¶, Pascal Ruffieux†, Xinliang Feng*§, and Roman Fasel*†‡

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b09212
28 Feb 08:22

[ASAP] Step-Growth Annulative p-Extension Polymerization for Synthesis of Cove-Type Graphene Nanoribbons

by Yuuta Yano†, Feijiu Wang†‡, Nobuhiko Mitoma†‡, Yuhei Miyauchi†‡§, Hideto Ito*†‡, and Kenichiro Itami*†‡?

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b11328
28 Feb 08:20

[ASAP] Solution Synthesis of Layered van der Waals (vdW) Ferromagnetic CrGeTe3 Nanosheets from a Non-vdW Cr2Te3Template

by Huan Yang†‡, Fang Wang*†‡, Huisheng Zhang‡, Lihong Guo†, Liyan Hu†‡, Lanfang Wang†‡, Ding-Jiang Xue*§, and Xiaohong Xu*†‡

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b13492
28 Feb 08:19

[ASAP] Aromatic Nanosandwich Obtained by s-Dimerization of a Nanographenoid p-Radical

by Liliia Moshniaha†, Marika Z?yla-Karwowska†, Piotr J. Chmielewski†, Tadeusz Lis†, Joanna Cybin´ska†‡, Elz?bieta Gon´ka†, Johannes Oschwald#, Thomas Drewello#, Samara Medina Rivero§, Juan Casado§, and Marcin Ste?pien´*†

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b13942
28 Feb 08:19

[ASAP] Single-Atom Vacancy Defect to Trigger High-Efficiency Hydrogen Evolution of MoS2

by Xin Wang#†‡, Yuwei Zhang#†‡, Haonan Si†‡, Qinghua Zhang§, Jing Wu†‡, Li Gao†‡, Xiaofu Wei†‡, Yu Sun†‡, Qingliang Liao†‡, Zheng Zhang†‡, Kausar Ammarah†‡, Lin Gu§??, Zhuo Kang*†‡, and Yue Zhang*†‡

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b12113
28 Feb 08:18

[ASAP] Ab Initio Molecular Dynamics of CdSe Quantum-Dot-Doped Glasses

by Wenke Li†‡, Xiujian Zhao†, Chao Liu*†, and Franc¸ois-Xavier Coudert*‡

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b12073
28 Feb 08:18

[ASAP] Cation Engineering in Two-Dimensional Ruddlesden–Popper Lead Iodide Perovskites with Mixed Large A-Site Cations in the Cages

by Yongping Fu†$, Xinyi Jiang†$, Xiaotong Li†, Boubacar Traore#§, Ioannis Spanopoulos†, Claudine Katan#, Jacky Even§, Mercouri G. Kanatzidis†, and Elad Harel*††

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b13587
17 Feb 00:00

Gapless ground state in the archetypal quantum kagome antiferromagnet ZnCu3(OH)6Cl2

by P. Khuntia

Nature Physics, Published online: 17 February 2020; doi:10.1038/s41567-020-0792-1

Herbertsmithite is an experimental realization of the so-called quantum kagome antiferromagnet, a system that is predicted to host a spin liquid state down to zero temperature. Detailed NMR measurements now confirm that this is the case, and that its ground state is indeed gapless.
09 Jan 09:01

[ASAP] Modular Design via Multiple Anion Chemistry of the High Mobility van der Waals Semiconductor Bi4O4SeCl2

by Quinn D. Gibson†, Troy D. Manning†, Marco Zanella†, Tianqi Zhao‡, Philip A. E. Murgatroyd§, Craig M. Robertson†, Leanne A. H. Jones§, Fiona McBride†, Rasmita Raval†, Furio Cora‡, Ben Slater‡, John B. Claridge†, Vin R. Dhanak§, Matthew S. Dyer†, Jonathan Alaria§, and Matthew J. Rosseinsky*†

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b09411
09 Jan 09:00

Nanoscale imaging of equilibrium quantum Hall edge currents and of the magnetic monopole response in graphene

by Aviram Uri

Nature Physics, Published online: 23 December 2019; doi:10.1038/s41567-019-0713-3

The microscopic quantum Hall edge currents and the equilibrium currents that generate the mirror magnetic monopoles in time-reversal-symmetry-broken topological matter are directly imaged in the quantum Hall state in graphene by using a SQUID-on-tip.
09 Jan 09:00

Correlated insulator by the slice

by Katharina J. Franke

Nature Physics, Published online: 06 January 2020; doi:10.1038/s41567-019-0760-9

A layer-by-layer study of TaSe2 shows how this material becomes increasingly insulating as it thins to a monolayer. Scanning tunnelling microscopy reveals the electronic correlations underlying this insulator with atomic resolution.
09 Jan 09:00

Strong correlations and orbital texture in single-layer 1T-TaSe2

by Yi Chen

Nature Physics, Published online: 06 January 2020; doi:10.1038/s41567-019-0744-9

The electrons that contribute to the Mott insulator state in single-layer 1T-TaSe2 are shown to also have a rich variation in their orbital occupation. As more layers are added, both the insulating state and orbital texture weaken.
21 Dec 05:40

[ASAP] The Green Box: An Electronically Versatile Perylene Diimide Macrocyclic Host for Fullerenes

by Timothy A. Barendt*†, William K. Myers‡, Stuart P. Cornes§, Maria A. Lebedeva†§, Kyriakos Porfyrakis§?, Igor Marques?, Vi´tor Fe´lix?, and Paul D. Beer*†

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b10929
21 Dec 05:37

[ASAP] Importance of Size and Contact Structure of Gold Nanoparticles for the Genesis of Unique Catalytic Processes

by Tamao Ishida*†‡, Toru Murayama†‡, Ayako Taketoshi†‡, and Masatake Haruta*‡

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Chemical Reviews
DOI: 10.1021/acs.chemrev.9b00551
21 Dec 05:35

Crossover from two-dimensional to three-dimensional superconducting states in bismuth-based cuprate superconductor

by Jing Guo

Nature Physics, Published online: 16 December 2019; doi:10.1038/s41567-019-0740-0

Applying pressure to a cuprate reveals that the strange metal phase has a two-dimensional character, as shown by emerging Berezinskii–Kosterlitz–Thouless behaviour.
21 Dec 05:35

Solids of quantum Hall skyrmions in graphene

by H. Zhou

Nature Physics, Published online: 16 December 2019; doi:10.1038/s41567-019-0729-8

The authors use spin waves to demonstrate that charged quantum Hall skyrmions exist away from integer filling. They also see evidence of several fractional skyrmion states.
09 Dec 02:48

[ASAP] Fullerene-Based Switching Molecular Diodes Controlled by Oriented External Electric Fields

by Adam Jaros?#†‡, Esmaeil Farajpour Bonab#§?, Michal Straka*†, and Cina Foroutan-Nejad*§??

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b07215
09 Dec 02:44

[ASAP] Nanoscale Phenomena in Lithium-Ion Batteries

by Sung-Kyun Jung†‡?, Insang Hwang†?, Donghee Chang†?, Kyu-Young Park†?, Sung Joo Kim†, Won Mo Seong†, Donggun Eum†, Jooha Park†, Byunghoon Kim†, Jihyeon Kim†, Jae Hoon Heo†, and Kisuk Kang*†‡§

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Chemical Reviews
DOI: 10.1021/acs.chemrev.9b00405
09 Dec 02:43

A magnetic field boost for superconductors

by Marc Janoschek

Nature Physics, Published online: 02 December 2019; doi:10.1038/s41567-019-0731-1

High-magnetic-field experiments on the recently discovered unconventional superconductor UTe2 are consistent with p-wave pairing arising while time-reversal symmetry is broken. In turn, this suggests that this material is a candidate for a chiral superconductor that may be exploited for topological quantum computing.
02 Dec 02:44

[ASAP] Molecular Control of Heterogeneous Electrocatalysis through Graphite Conjugation

by Megan N. Jackson† and Yogesh Surendranath*

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Accounts of Chemical Research
DOI: 10.1021/acs.accounts.9b00439
02 Dec 02:43

[ASAP] Large Thermal Conductivity Drops in the Diamondoid Lattice of CuFeS2 by Discordant Atom Doping

by Hongyao Xie†‡, Xianli Su*†, Shiqiang Hao§, Cheng Zhang†, Zhengkai Zhang†, Wei Liu†, Yonggao Yan†, Christopher Wolverton§, Xinfeng Tang*†, and Mercouri G. Kanatzidis*‡

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b10983
02 Dec 02:42

[ASAP] Pocketlike Active Site of Rh1/MoS2 Single-Atom Catalyst for Selective Crotonaldehyde Hydrogenation

by Yang Lou†‡, Yongping Zheng§?, Xu Li†, Na Ta†, Jia Xu†, Yifan Nie§, Kyeongjae Cho*§, and Jingyue Liu*†

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b06628
02 Dec 02:40

[ASAP] Direct Observation of Symmetry-Dependent Electron–Phonon Coupling in Black Phosphorus

by Nannan Mao†‡?, Xingzhi Wang‡§?, Yuxuan Lin†, Bobby G. Sumpter?#, Qingqing Ji†, Toma´s Palacios†, Shengxi Huang?, Vincent Meunier?, Mildred S. Dresselhaus†, William A. Tisdale?, Liangbo Liang*?, Xi Ling*‡§¶, and Jing Kong*†

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b07974
02 Dec 02:39

[ASAP] A New Three-Dimensional Subsulfide Ir2In8S with Dirac Semimetal Behavior

by Jason F. Khoury†, Alexander J. E. Rettie‡§, Mojammel A. Khan‡, Nirmal J. Ghimire‡?, In~igo Robredo??, Jonathan E. Pfluger#, Koushik Pal#, Chris Wolverton#, Aitor Bergara???, J. S. Jiang‡, Leslie M. Schoop¶, Maia G. Vergniory??, J. F. Mitchell‡, Duck Young Chung‡, and Mercouri G. Kanatzidis*†‡

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b10147
02 Dec 02:38

[ASAP] Cobalt-Modulated Molybdenum–Dinitrogen Interaction in MoS2 for Catalyzing Ammonia Synthesis

by Jing Zhang†?, Xiaoyin Tian†?, Mingjie Liu*‡, Hua Guo†, Jiadong Zhou§, Qiyi Fang†, Zheng Liu§, Qin Wu‡, and Jun Lou*†

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b02501
02 Dec 02:37

[ASAP] Frustrated and Allowed Structural Transitions: The Theory-Guided Discovery of the Modulated Structure of IrSi

by Hillary E. Mitchell Warden and Daniel C. Fredrickson*

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b10473
12 Nov 01:34

[ASAP] Two-Dimensional Organic–Inorganic Perovskite Ferroelectric Semiconductors with Fluorinated Aromatic Spacers

by Ping-Ping Shi†, Si-Qi Lu†, Xian-Jiang Song†, Xiao-Gang Chen†, Wei-Qiang Liao*‡, Peng-Fei Li‡, Yuan-Yuan Tang*‡, and Ren-Gen Xiong*†‡

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b10048
12 Nov 01:32

[ASAP] Structural and Electronic Optimization of MoS2 Edges for Hydrogen Evolution

by Hao Wang†‡¶, Xu Xiao§¶, Shuyuan Liu†¶, Chao-Lung Chiang?, Xiaoxiao Kuai†, Chun-Kuo Peng??, Yu-Chang Lin??, Xing Meng§#, Jianqing Zhao†, Jinho Choi*†, Yan-Gu Lin?, Jong-Min Lee*‡, and Lijun Gao*†

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Journal of the American Chemical Society
DOI: 10.1021/jacs.9b09932