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08 Jun 02:08

Stacking Domains and Dislocation Networks in Marginally Twisted Bilayers of Transition Metal Dichalcogenides

by V. V. Enaldiev, V. Zólyomi, C. Yelgel, S. J. Magorrian, and V. I. Fal’ko

Author(s): V. V. Enaldiev, V. Zólyomi, C. Yelgel, S. J. Magorrian, and V. I. Fal’ko

We apply a multiscale modeling approach to study lattice reconstruction in marginally twisted bilayers of transition metal dichalcogenides (TMD). For this, we develop density functional theory parametrized interpolation formulae for interlayer adhesion energies of MoSe2, WSe2, MoS2, and WS2, combine...


[Phys. Rev. Lett. 124, 206101] Published Wed May 20, 2020

25 May 08:28

Two-dimensional stable Mn based half metal and antiferromagnets promising for spintronics

Nanoscale, 2020, 12,12490-12496
DOI: 10.1039/D0NR03526B, Paper
Bingwen Zhang, Guang Song, Jie Sun, Jiancai Leng, Cheng Zhang, Jun Wang
By phonon band structure calculations and Monte Carlo simulations, we propose that 2D MnSi and MnC0.5Si0.5 monolayers could exhibit mechanical stability and room temperature half-metallic properties.
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25 May 08:24

Superconductivity and strong correlations in moiré flat bands

by Leon Balents

Nature Physics, Published online: 19 May 2020; doi:10.1038/s41567-020-0906-9

The identification of superconductivity and strong interactions in twisted bilayer 2D materials prompted many questions about the interplay of these phenomena. This Perspective presents the status of the field and the urgent issues for future study.
25 May 08:23

The interplay between thermodynamics and kinetics in the solid-state synthesis of layered oxides

by Matteo Bianchini

Nature Materials, Published online: 18 May 2020; doi:10.1038/s41563-020-0688-6

Understanding the competition between thermodynamics and kinetics is crucial for the rational synthesis of inorganic materials. The synthesis of two-layer sodium metal oxides is investigated by in situ synchrotron XRD and a model is developed to rationalize why the observed phase progression proceeds through non-equilibrium three-layered intermediates.
25 May 08:23

Making 2D topological polymers a reality

by Yu Jing

Nature Materials, Published online: 18 May 2020; doi:10.1038/s41563-020-0690-z

First-principles calculations predicted electronic topological properties for 2D honeycomb–kagome polymers, which have been now confirmed experimentally thanks to improvements in on-surface synthesis.
25 May 08:22

Author Correction: Axionic charge-density wave in the Weyl semimetal (TaSe4)2I

by J. Gooth

Nature, Published online: 15 May 2020; doi:10.1038/s41586-020-2303-z

Author Correction: Axionic charge-density wave in the Weyl semimetal (TaSe4)2I
25 May 08:14

Transition metal ditellurides make for better 2D contacts

by Wei Liu

Nature Electronics, Published online: 13 April 2020; doi:10.1038/s41928-020-0403-2

Metal–semiconductor junctions formed between a transition metal ditelluride and monolayer molybdenum disulfide exhibit nearly ideal Schottky–Mott conditions.
19 May 03:25

Two-dimensional nanocoating-enabled orthopedic implants for bimodal therapeutic applications

Nanoscale, 2020, 12,11936-11946
DOI: 10.1039/D0NR02327B, Paper
Song Wang, Chunyan Duan, Weizhong Yang, Xiangyu Gao, Jiacheng Shi, Jianping Kang, Yi Deng, Xiao-Lei Shi, Zhi-Gang Chen
A multifunctional two-dimensional nanocoating consists of graphene oxide nanosheets, polydopamine nanofilm, and oligopeptide constructed on porous sulfonated polyetheretherketone for the purpose of bone infection treatment.
The content of this RSS Feed (c) The Royal Society of Chemistry
19 May 03:24

The alignment-dependent properties and applications of graphene moiré superstructures on the Ru(0001) surface

Nanoscale, 2020, 12,12831-12839
DOI: 10.1039/D0NR02370A, Paper
Leining Zhang, Jichen Dong, Zhaoyong Guan, Xiuyun Zhang, Feng Ding
The moiré superstructure of graphene on a lattice-mismatched metal substrate has profound effects on the electronic properties of graphene and can be used for many applications.
The content of this RSS Feed (c) The Royal Society of Chemistry
19 May 03:24

Hybridized intervalley moiré excitons and flat bands in twisted WSe2 bilayers

Nanoscale, 2020, 12,11088-11094
DOI: 10.1039/D0NR02160A, Paper
Open Access Open Access
Samuel Brem, Kai-Qiang Lin, Roland Gillen, Jonas M. Bauer, Janina Maultzsch, John M. Lupton, Ermin Malic
Twisted WSe2 bilayers exhibit hybridized K–Λ excitons with flat moiré bands, which become visible through phonon-assisted photoluminescence.
The content of this RSS Feed (c) The Royal Society of Chemistry
19 May 03:24

Solution-gated transistors of two-dimensional materials for chemical and biological sensors: status and challenges

Nanoscale, 2020, 12,11364-11394
DOI: 10.1039/D0NR01125H, Review Article
Qin Fan, Lude Wang, Duo Xu, Yanhong Duo, Jie Gao, Lei Zhang, Xianbao Wang, Xiang Chen, Jinhua Li, Han Zhang
Two-dimensional materials are widely used in solution-gated transistors for biochemical sensing due to their excellent properties and large specific surface area.
The content of this RSS Feed (c) The Royal Society of Chemistry
19 May 03:24

Multi-component (Ag–Au–Cu–Pd–Pt) alloy nanoparticle-decorated p-type 2D-molybdenum disulfide (MoS2) for enhanced hydrogen sensing

Nanoscale, 2020, 12,11830-11841
DOI: 10.1039/D0NR02177F, Communication
Kusuma M. B. Urs, Nirmal Kumar Katiyar, Ritesh Kumar, Krishanu Biswas, Abhishek K. Singh, C. S. Tiwary, Vinayak Kamble
The nanoscale interface between multi-component (Ag–Au–Cu–Pd–Pt) alloy nanoparticles on MoS2 sheets increase its work function making an ohmic contact into Schottky with gold electrodes. This drastically enhances response towards hydrogen gas.
The content of this RSS Feed (c) The Royal Society of Chemistry
19 May 03:23

Twistronics in tensile strained bilayer black phosphorus

Nanoscale, 2020, 12,12909-12916
DOI: 10.1039/D0NR02179B, Paper
Peng Kang, Wanting Zhang, Vincent Michaud-Rioux, Xin Wang, Jiangni Yun, Hong Guo
A study of the electronic and mechanical properties of tensile strained twisted bilayer black phosphorus.
The content of this RSS Feed (c) The Royal Society of Chemistry
19 May 03:23

A polyimide-pyrolyzed carbon waste approach for the scalable and controlled electrochemical preparation of size-tunable graphene

Nanoscale, 2020, 12,11971-11978
DOI: 10.1039/D0NR00725K, Paper
Haoguang Huang, Li Peng, Wenzhang Fang, Shengying Cai, Xingyuan Chu, Yingjun Liu, Weiwei Gao, Zhen Xu, Chao Gao
The industrial carbon wastes are converted to be size-tunable graphene and GQDs with high yield.
The content of this RSS Feed (c) The Royal Society of Chemistry
19 May 03:21

2D materials beyond graphene toward Si integrated infrared optoelectronic devices

Nanoscale, 2020, 12,11784-11807
DOI: 10.1039/D0NR02574G, Review Article
Changyong Lan, Zhe Shi, Rui Cao, Chun Li, Han Zhang
A study of typical 2D materials beyond graphene suitable for infrared applications, in particular, infrared light emitting devices, optical modulators, and photodetectors.
The content of this RSS Feed (c) The Royal Society of Chemistry
19 May 03:21

Large excitonic effect on van der Waals interaction between two-dimensional semiconductors

Nanoscale, 2020, 12,12639-12646
DOI: 10.1039/D0NR02152K, Paper
Jiabao Yang, Xiaofei Liu, Wanlin Guo
Electron–hole interaction has an exceptionally large effect on the long-range van der Waals energy between two-dimensional semiconductors.
The content of this RSS Feed (c) The Royal Society of Chemistry
19 May 03:19

[ASAP] Pressure Manipulation of Interlayer Interactions and Ultrafast Carrier Dynamics in Few-Layer MoS2

by Qingyi Li†‡, Laizhi Sui‡, Guangming Niu‡, Jutao Jiang‡, Yutong Zhang‡, Guorong Wu‡, Mingxing Jin*†, and Kaijun Yuan*‡

TOC Graphic

The Journal of Physical Chemistry C
DOI: 10.1021/acs.jpcc.0c01869
19 May 03:19

[ASAP] Anisotropic Atomic Mobilities of Layer-Structured O3 LixCoO2 Cathodes and Their Applications in Optimization of Battery Performance

by Fangzhou Xing, Sa Ma, and Lijun Zhang*

TOC Graphic

The Journal of Physical Chemistry C
DOI: 10.1021/acs.jpcc.0c01946
19 May 03:18

[ASAP] Origin of Confined Catalysis in Nanoscale Reactors between Two-Dimensional Covers and Metal Substrates: Mechanical or Electronic?

by Fenfei Wei†, Qiang Wan†, Sen Lin*†, and Hua Guo*‡

TOC Graphic

The Journal of Physical Chemistry C
DOI: 10.1021/acs.jpcc.0c03621
19 May 03:17

[ASAP] Ultrafast Spin Crossover in a Room-Temperature Ferrimagnet: Element-Specific Spin Dynamics in Photoexcited Cobalt Ferrite

by Stephen Londo†, Somnath Biswas†, Jakub Husek†, Igor V. Pinchuk‡, Michael J. Newburger‡, Alexandra Boyadzhiev‡, Amanda H. Trout¶§, David W. McComb¶§, Roland Kawakami‡, and L. Robert Baker*†

TOC Graphic

The Journal of Physical Chemistry C
DOI: 10.1021/acs.jpcc.0c03736
19 May 03:17

[ASAP] Isomers Matter: Physicochemical Properties Dictated by the Position of S and Se in Single Layer MoSSe

by Muthu Austeria P*, P Vinoth Babu, and S. Sampath*

TOC Graphic

The Journal of Physical Chemistry C
DOI: 10.1021/acs.jpcc.0c01516
19 May 03:17

[ASAP] Efficient Ab Initio Modeling of Dielectric Screening in 2D van der Waals Materials: Including Phonons, Substrates, and Doping

by M. N. Gjerding*†‡, L. S. R. Cavalcante§, Andrey Chaves§?, and K. S. Thygesen†‡

TOC Graphic

The Journal of Physical Chemistry C
DOI: 10.1021/acs.jpcc.0c01635
19 May 03:14

Synthesis of mesoscale ordered two-dimensional π-conjugated polymers with semiconducting properties

by G. Galeotti

Nature Materials, Published online: 18 May 2020; doi:10.1038/s41563-020-0682-z

Optimized Ullmann coupling reaction of heterotriangulene precursors allows the synthesis of two-dimensional π-conjugated polymers with ordered domains larger than 100 × 100 nm2 showing both Dirac cones and flat bands in their electronic structure.
19 May 03:11

Engineering covalently bonded 2D layered materials by self-intercalation

by Xiaoxu Zhao

Nature, Published online: 13 May 2020; doi:10.1038/s41586-020-2241-9

The intercalation of native atoms into bilayer transition metal dichalcogenides during growth generates ultrathin, covalently bonded materials into which ferromagnetic ordering can be introduced.
12 May 01:10

[ASAP] Strain and Piezo-Doping Mismatch between Graphene Layers

by Alexis Forestier†, Fe´lix Balima†, Colin Bousige*‡, Garde^nia de Sousa Pinheiro†§, Re´my Fulcrand†, Martin Kalba´c??, Denis Machon*†?, and Alfonso San-Miguel*†

TOC Graphic

The Journal of Physical Chemistry C
DOI: 10.1021/acs.jpcc.0c01898
12 May 01:10

[ASAP] Formation of Hexagonal PdSe2 for Electronics and Catalysis

by Zhenhua Wu†, Lei Lu‡§, Xiaochong Liang?, Chaochao Dun?, Shicheng Yan§, Erzhen Mu†, Yang Liu†, and Zhiyu Hu*†

TOC Graphic

The Journal of Physical Chemistry C
DOI: 10.1021/acs.jpcc.0c00521
12 May 01:07

An ultrathin two-dimensional vertical ferroelectric tunneling junction based on CuInP2S6 monolayer

Nanoscale, 2020, 12,12522-12530
DOI: 10.1039/D0NR01475C, Paper
Min Zhao, Gaoyang Gou, Xiangdong Ding, Jun Sun
A 1 nm-thick 2D vertical ferroelectric tunneling junction composed of a van der Waals stacked graphene/CuInP2S6 monolayer/graphene heterostructure.
The content of this RSS Feed (c) The Royal Society of Chemistry
12 May 01:06

Charge doping induced reversible multistep structural phase transitions and electromechanical actuation in two-dimensional 1T′-MoS2

Nanoscale, 2020, 12,12541-12550
DOI: 10.1039/D0NR02049D, Paper
Kaiyun Chen, Junkai Deng, Qian Shi, Xiangdong Ding, Jun Sun, Sen Yang, Jefferson Zhe Liu
Charge doping could effectively modulate the charge density wave state of monolayer MoS2 with large strain output and superelasticity.
The content of this RSS Feed (c) The Royal Society of Chemistry
12 May 01:04

Twist-angle-dependent interlayer exciton diffusion in WS2–WSe2 heterobilayers

by Long Yuan

Nature Materials, Published online: 11 May 2020; doi:10.1038/s41563-020-0670-3

Interlayer exciton dynamics in a van der Waals heterostructure is found to be modulated by the twist angle between the atomically thin layers, elucidating the effect of moiré potentials on exciton motion and providing guidelines to design quantum photonics devices based on 2D materials.
12 May 01:02

Mapping the twist-angle disorder and Landau levels in magic-angle graphene

by A. Uri

Nature, Published online: 06 May 2020; doi:10.1038/s41586-020-2255-3

SQUID-on-tip tomographic imaging of Landau levels in magic-angle graphene provides nanoscale maps of local twist-angle disorder and shows that its properties are fundamentally different from common types of disorder.