Shared posts

18 Jan 01:10

Atomically precise single-crystal structures of electrically conducting 2D metal–organic frameworks

by Jin-Hu Dou

Nature Materials, Published online: 23 November 2020; doi:10.1038/s41563-020-00847-7

Two-dimensional MOFs can possess porosity and electrical conductivity but are difficult to grow as single crystals. Here, by balancing in-plane and out-of-plane interactions, single crystals of sizes up to 200 µm are grown, allowing in-plane transport measurements and atomic-resolution analysis.
29 Dec 07:22

In situ imaging of two-dimensional surface growth reveals the prevalence and role of defects in zeolite crystallization [Chemistry]

by Madhuresh K. Choudhary, Rishabh Jain, Jeffrey D. Rimer
Zeolite crystallization predominantly occurs by nonclassical pathways involving the attachment of complex (alumino)silicate precursors to crystal surfaces, yet recurrent images of fully crystalline materials with layered surfaces are evidence of classical growth by molecule attachment. Here we use in situ atomic force microscopy to monitor three distinct mechanisms of two-dimensional...
21 Dec 05:56

A metal–organic framework that exhibits CO2-induced transitions between paramagnetism and ferrimagnetism

by Jun Zhang

Nature Chemistry, Published online: 30 November 2020; doi:10.1038/s41557-020-00577-y

Metal–organic frameworks (MOFs) can combine porosity and magnetic order within their lattice, which makes them attractive for the development of stimuli-responsive magnets. Now, a MOF has been prepared that converts from a ferrimagnet to a paramagnet with CO2 uptake, and returns to the ferrimagnetic state on releasing CO2.
15 Dec 13:07

Graphene bilayers with a twist

by Eva Y. Andrei

Nature Materials, Published online: 18 November 2020; doi:10.1038/s41563-020-00840-0

Magic-angle twisted bilayer graphene plays host to many interesting phenomena, including superconductivity. This Review highlights key research results in the field, points toward important open questions, and comments on the place of magic-angle twisted bilayer graphene in the strongly correlated quantum matter world.
11 Dec 01:26

[ASAP] Two-Dimensional Silicon/Carbon from Commercial Alloy and CO2 for Lithium Storage and Flexible Ti3C2Tx MXene-Based Lithium–Metal Batteries

by Yongling An, Yuan Tian, Yuchan Zhang, Chuanliang Wei, Liwen Tan, Chenghui Zhang, Naxin Cui, Shenglin Xiong, Jinkui Feng, and Yitai Qian

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ACS Nano
DOI: 10.1021/acsnano.0c08336
11 Dec 01:25

[ASAP] Kinetics-Limited Two-Step Growth of van der Waals Puckered Honeycomb Sb Monolayer

by Zhi-Qiang Shi, Huiping Li, Qian-Qian Yuan, Cheng-Long Xue, Yong-Jie Xu, Yang-Yang Lv, Zhen-Yu Jia, Yanbin Chen, Wenguang Zhu, and Shao-Chun Li

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ACS Nano
DOI: 10.1021/acsnano.0c04620
11 Dec 01:24

[ASAP] Defect-Induced in Situ Atomic Doping in Transition Metal Dichalcogenides via Liquid-Phase Synthesis toward Efficient Electrochemical Activity

by Junghyun Lee, Jungwoo Heo, Hyeong Yong Lim, Jihyung Seo, Youngwoo Kim, Jihyun Kim, Ungsoo Kim, Yunseong Choi, Su Hwan Kim, Yung Jin Yoon, Tae Joo Shin, Joohoon Kang, Sang Kyu Kwak, Jin Young Kim, and Hyesung Park

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ACS Nano
DOI: 10.1021/acsnano.0c06783
11 Dec 01:23

[ASAP] Direct Bandgap-like Strong Photoluminescence from Twisted Multilayer MoS2 Grown on SrTiO3

by Soumya Sarkar, Sinu Mathew, Sandhya Chintalapati, Ashutosh Rath, Majid Panahandeh-Fard, Surajit Saha, Sreetosh Goswami, Sherman Jun Rong Tan□, Kian Ping Loh□, Mary Scott■, and Thirumalai Venkatesan△▽

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ACS Nano
DOI: 10.1021/acsnano.0c04801
11 Dec 01:21

Exchange bias switching in an antiferromagnet/ferromagnet bilayer driven by spin–orbit torque

by Shouzhong Peng

Nature Electronics, Published online: 30 November 2020; doi:10.1038/s41928-020-00504-6

The magnetization and exchange bias field in an IrMn/CoFeB bilayer can be independently switched using a current-controlled spin–orbit torque generated in the antiferromagnetic IrMn layer.
11 Dec 01:19

Two-dimensional transistors with reconfigurable polarities for secure circuits

by Peng Wu

Nature Electronics, Published online: 07 December 2020; doi:10.1038/s41928-020-00511-7

Transistors that use two-dimensional black phosphorus as the active material can dynamically switch between p-type and n-type operation, and can be used to create security primitive circuits with polymorphic NAND/NOR obfuscation functionality.
03 Dec 11:21

[ASAP] Metalated Graphyne-Based Networks as Two-Dimensional Materials: Crystallization, Topological Defects, Delocalized Electronic States, and Site-Specific Doping

by Zechao Yang, Tim Sander, Julian Gebhardt, Tobias A. Schaub, Jörg Schönamsgruber, Himadri R. Soni, Andreas Görling, Milan Kivala, and Sabine Maier

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ACS Nano
DOI: 10.1021/acsnano.0c05865
03 Dec 11:19

[ASAP] Formation of Coherent 1H–1T Heterostructures in Single-Layer MoS2 on Au(111)

by Fanglue Wu, Zhuotong Liu, Nathaniel Hawthorne, Michael Chandross, Quentarius Moore, Nicolas Argibay, John F. Curry, and James D. Batteas

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ACS Nano
DOI: 10.1021/acsnano.0c06014
03 Dec 11:12

Publisher Correction: Room-temperature superconductivity in a carbonaceous sulfur hydride

by Elliot Snider

Nature, Published online: 20 November 2020; doi:10.1038/s41586-020-2955-8

Publisher Correction: Room-temperature superconductivity in a carbonaceous sulfur hydride
03 Dec 11:12

Unconventional ferroelectricity in moiré heterostructures

by Zhiren Zheng

Nature, Published online: 23 November 2020; doi:10.1038/s41586-020-2970-9

Electronic ferroelectricity is observed in a graphene-based moiré heterostructure, which is explained using a spontaneous interlayer charge-transfer model driven by layer-specific on-site Coulomb repulsion.
23 Nov 01:36

[ASAP] Free-Standing Two-Dimensional Gold Membranes Produced by Extreme Mechanical Thinning

by Qi Zhu, Youran Hong, Guang Cao, Yin Zhang, Xiaohan Zhang, Kui Du, Ze Zhang, Ting Zhu, and Jiangwei Wang

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ACS Nano
DOI: 10.1021/acsnano.0c06697
23 Nov 01:34

[ASAP] Mechanisms and Applications of Steady-State Photoluminescence Spectroscopy in Two-Dimensional Transition-Metal Dichalcogenides

by Mike Tebyetekerwa, Jian Zhang, Zhen Xu, Thien N. Truong, Zongyou Yin, Yuerui Lu, Seeram Ramakrishna, Daniel Macdonald, and Hieu T. Nguyen

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ACS Nano
DOI: 10.1021/acsnano.0c08668
23 Nov 01:31

[ASAP] Direct Measurement of Folding Angle and Strain Vector in Atomically Thin WS2 Using Second-Harmonic Generation

by Ahmed Raza Khan, Boqing Liu, Tieyu Lü, Linglong Zhang, Ankur Sharma, Yi Zhu, Wendi Ma, and Yuerui Lu

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ACS Nano
DOI: 10.1021/acsnano.0c06901
23 Nov 01:30

[ASAP] Chiral Bilayer All-Dielectric Metasurfaces

by Katsuya Tanaka, Dennis Arslan, Stefan Fasold, Michael Steinert, Jürgen Sautter, Matthias Falkner, Thomas Pertsch, Manuel Decker, and Isabelle Staude■

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ACS Nano
DOI: 10.1021/acsnano.0c07295
23 Nov 01:30

[ASAP] 2H-MoS2 on Mo2CTx MXene Nanohybrid for Efficient and Durable Electrocatalytic Hydrogen Evolution

by Kang Rui Garrick Lim, Albertus D. Handoko, Luke R. Johnson, Xing Meng, Ming Lin, Gomathy Sandhya Subramanian, Babak Anasori, Yury Gogotsi, Aleksandra Vojvodic, and Zhi Wei Seh

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ACS Nano
DOI: 10.1021/acsnano.0c08671
23 Nov 01:29

[ASAP] Ultrabroadband Tuning and Fine Structure of Emission Spectra in Lanthanide Er-Doped ZnSe Nanosheets for Display and Temperature Sensing

by Yuan Liu, Gongxun Bai, Yongxin Lyu, Youjie Hua, Renguang Ye, Junjie Zhang, Liang Chen, Shiqing Xu, and Jianhua Hao

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ACS Nano
DOI: 10.1021/acsnano.0c07547
23 Nov 01:28

[ASAP] Photophysics and Electronic Structure of Lateral Graphene/MoS2 and Metal/MoS2 Junctions

by Shruti Subramanian, Quinn T. Campbell, Simon K. Moser, Jonas Kiemle, Philipp Zimmermann, Paul Seifert, Florian Sigger, Deeksha Sharma⊙, Hala Al-Sadeg, Michael Labella, III◊, Dacen Waters◨, Randall M. Feenstra◨, Roland J. Koch, Chris Jozwiak, Aaron Bostwick, Eli Rotenberg, Ismaila Dabo, Alexander W. Holleitner, Thomas E. Beechem◓, Ursula Wurstbauer⧫, and Joshua A. Robinson◪⊕

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ACS Nano
DOI: 10.1021/acsnano.0c02527
23 Nov 01:26

[ASAP] Inclined Ultrathin Bi2O2Se Films: A Building Block for Functional van der Waals Heterostructures

by Chengyun Hong, Ye Tao, Anmin Nie, Minhao Zhang, Nan Wang, Ruiping Li, Junquan Huang, Yongqing Huang, Xiaomin Ren, Yingchun Cheng, and Xiaolong Liu

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ACS Nano
DOI: 10.1021/acsnano.0c05300
23 Nov 01:26

[ASAP] Ultrasensitive Magnetic Sensors Enabled by Heterogeneous Integration of Graphene Hall Elements and Silicon Processing Circuits

by Tongyu Dai, Chengying Chen, Le Huang, Jianhua Jiang, Lian-Mao Peng, and Zhiyong Zhang

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ACS Nano
DOI: 10.1021/acsnano.0c08435
23 Nov 01:25

[ASAP] Tuning the Band Structure of MoS2 via Co9S8@MoS2 Core–Shell Structure to Boost Catalytic Activity for Lithium–Sulfur Batteries

by Boyu Li, Qingmei Su, Lintao Yu, Jun Zhang, Gaohui Du, Dong Wang, Di Han, Miao Zhang, Shukai Ding, and Bingshe Xu

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ACS Nano
DOI: 10.1021/acsnano.0c07332
23 Nov 01:25

[ASAP] cm2-Scale Synthesis of MoTe2 Thin Films with Large Grains and Layer Control

by David J. Hynek, Raivat M. Singhania, Shiyu Xu, Benjamin Davis, Leizhi Wang, Milad Yarali, Joshua V. Pondick, John M. Woods, Nicholas C. Strandwitz, and Judy J. Cha

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ACS Nano
DOI: 10.1021/acsnano.0c08069
23 Nov 01:25

[ASAP] Scalable Integration of Coplanar Heterojunction Monolithic Devices on Two-Dimensional In2Se3

by Subhrajit Mukherjee, Debopriya Dutta, Pranab K. Mohapatra, Lital Dezanashvili, Ariel Ismach, and Elad Koren

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ACS Nano
DOI: 10.1021/acsnano.0c08146
16 Nov 01:31

Picosecond switching in a ferromagnet

by Can Onur Avci

Nature Electronics, Published online: 09 November 2020; doi:10.1038/s41928-020-00502-8

An ultrashort pulse of electric current can be used to switch the magnetization of a micrometre-scale magnetic element via spin–orbit torques.
16 Nov 01:31

Two-dimensional Ruddlesden–Popper layered perovskite solar cells based on phase-pure thin films

by Chao Liang

Nature Energy, Published online: 09 November 2020; doi:10.1038/s41560-020-00721-5

Two-dimensional Ruddlesden–Popper layered metal-halide perovskites show better performance over three-dimensional versions, but are typically based on quantum wells with random width distribution. Liang et al. show that introducing molten salt spacers gives phase-pure quantum wells and improved solar cell performance.
16 Nov 01:30

Observation of single-defect memristor in an MoS2 atomic sheet

by Saban M. Hus

Nature Nanotechnology, Published online: 09 November 2020; doi:10.1038/s41565-020-00789-w

A combination of atomistic imaging and spectroscopy reveals that metal substitution into a sulfur vacancy is the underlying mechanism for resistive switching in transition metal dichalcogenide monolayers.
16 Nov 01:29

 Anatomy of cage formation in a two-dimensional glass-forming liquid

by Bo Li

Nature, Published online: 11 November 2020; doi:10.1038/s41586-020-2869-5

The onset of rigidity in a two-dimensional colloidal glass-forming system is identified by the formation and merging of locally rigid domains in which particles move in a cooperative manner.