Shared posts

07 Nov 03:11

[ASAP] Two-Dimensional Wedge-Shaped Magnetic EuS: Insight into the Substrate Step-Guided Epitaxial Synthesis on Sapphire

by Biao Zhang, Chao Yun, Heng Wu, Zijing Zhao, Yi Zeng, Dong Liang, Tong Shen, Jine Zhang, Xiaoxiao Huang, Jiepeng Song, Junjie Xu, Qing Zhang, Ping-Heng Tan, Song Gao, and Yanglong Hou

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Journal of the American Chemical Society
DOI: 10.1021/jacs.2c06023
07 Nov 03:10

Spatially Resolved Polarization Manipulation of Ferroelectricity in Twisted hBN

by Ming Lv, Xinzuo Sun, Yan Chen, Takashi Taniguchi, Kenji Watanabe, Menghao Wu, Jianlu Wang, Jiamin Xue
Spatially Resolved Polarization Manipulation of Ferroelectricity in Twisted hBN

Ferroelectricity is generated in twisted hBN flakes, which are used as a ferroelectric tunneling junction. Spatially resolved investigation by a conductive atomic force microscope tip reveals the unconventional ferroelectricity in this system, including lattice-slide-induced domain change, an unusual relationship between the tunneling resistance and polarization, and highly spatially dependent ferroelectric hysteresis.


Abstract

Robust room-temperature interfacial ferroelectricity has been formed in the 2D limit by simply twisting two atomic layers of non-ferroelectric hexagonal boron nitride (hBN). A thorough understanding of this newly discovered ferroelectric system is required. Here, twisted hBN is used as a tunneling junction and it is studied at the nanometer scale using conductive atomic force microscopy. Three properties unique to this system are discovered. First, the polarization dependence of the tunneling resistance contrasts with the conventional theory. Second, the ferroelectric domains can be controlled using mechanical stress, highlighting the original meaning of the emergent “slidetronics”. Third, ferroelectric hysteresis is highly spatially dependent. The hysteresis is symmetric at the domain walls. A few nanometers away, the hysteresis shifts completely to the positive or negative side, depending on the original polarization. These findings reveal the unconventional ferroelectricity in this 2D system.

07 Nov 02:59

Field-induced ultrafast modulation of Rashba coupling at room temperature in ferroelectric α-GeTe(111)

by Geoffroy Kremer

Nature Communications, Published online: 27 October 2022; doi:10.1038/s41467-022-33978-3

The ferroelectric material α-GeTe(111) is an excellent playground for spin-to charge conversion due to its strong Rashba coupling. Here, the authors reveal an ultrafast modulation of its Rashba coupling on the femtosecond timescale.
07 Nov 02:49

[ASAP] Electrical Gating of the Charge-Density-Wave Phases in Two-Dimensional h‑BN/1T-TaS2 Devices

by Maedeh Taheri, Jonas Brown, Adil Rehman, Nicholas Sesing, Fariborz Kargar, Tina T. Salguero, Sergey Rumyantsev, and Alexander A. Balandin

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ACS Nano
DOI: 10.1021/acsnano.2c07876
31 Oct 01:47

Heterojunction tunnel triodes based on two-dimensional metal selenide and three-dimensional silicon

by Jinshui Miao

Nature Electronics, Published online: 27 October 2022; doi:10.1038/s41928-022-00849-0

Gate-tunable heterojunction diodes—or triodes—that are based on van der Waals heterostructures formed from two-dimensional indium selenide and three-dimensional silicon can exhibit subthreshold slopes of 6.4 mV decade–1 and on-state current densities of 0.3 µA µm–1 at a drain bias of –1 V.
31 Oct 01:46

[ASAP] Exchange Bias State at the Crossover to 2D Ferromagnetism

by Dmitry V. Averyanov, Ivan S. Sokolov, Alexander N. Taldenkov, Oleg E. Parfenov, Igor A. Karateev, Oleg A. Kondratev, Andrey M. Tokmachev, and Vyacheslav G. Storchak

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ACS Nano
DOI: 10.1021/acsnano.2c09452
31 Oct 01:46

[ASAP] Interfacial Charge-Modulated Multifunctional MoS2/Ti3C2Tx Penetrating Electrode for High-Efficiency Freshwater Production

by Hantong Qie, Meng Liu, Xinping Fu, Xiao Tan, Yu Zhang, Meng Ren, Yinjie Zhang, Yuansheng Pei, Aijun Lin, Beidou Xi, and Jun Cui

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ACS Nano
DOI: 10.1021/acsnano.2c07810
31 Oct 01:45

[ASAP] Robust Bioinspired MXene–Hemicellulose Composite Films with Excellent Electrical Conductivity for Multifunctional Electrode Applications

by Ruwei Chen, Hao Tang, Yuhang Dai, Wei Zong, Wei Zhang, Guanjie He, and Xiaohui Wang

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ACS Nano
DOI: 10.1021/acsnano.2c08163
31 Oct 01:44

[ASAP] 2D Magnetic Semiconductor Fe3GeTe2 with Few and Single Layers with a Greatly Enhanced Intrinsic Exchange Bias by Liquid-Phase Exfoliation

by Suping Ma, Guanghao Li, Zhuo Li, Yawen Zhang, Haolin Lu, Zhansheng Gao, Jinxiong Wu, Guankui Long, and Yi Huang

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ACS Nano
DOI: 10.1021/acsnano.2c09143
31 Oct 01:44

[ASAP] Bifunctional Monolayer WSe2/Graphene Self-Stitching Heterojunction Microreactors for Efficient Overall Water Splitting in Neutral Medium

by Chun-Hao Chiang, Yueh-Chiang Yang, Jia-Wei Lin, Yung-Chang Lin, Po-Tuan Chen, Chung-Li Dong, Hung-Min Lin, Kwun Man Chan, Yu-Ting Kao, Kazu Suenaga, Po-Wen Chiu, and Chun-Wei Chen◇

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ACS Nano
DOI: 10.1021/acsnano.2c05986
31 Oct 01:44

[ASAP] High-Speed Transition-Metal Dichalcogenides Based Schottky Photodiodes for Visible and Infrared Light Communication

by Youwei Zhang, Wang Shen, Su Wu, Weijia Tang, Yantao Shu, Kankan Ma, Butian Zhang, Peng Zhou, and Shun Wang

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ACS Nano
DOI: 10.1021/acsnano.2c08394
31 Oct 01:43

A tunable monolithic SQUID in twisted bilayer graphene

by Elías Portolés

Nature Nanotechnology, Published online: 24 October 2022; doi:10.1038/s41565-022-01222-0

Twisting bilayer graphene to specific angles can yield correlated phases. A superconducting quantum interference device made from this magic-angle twisted bilayer graphene makes it possible to control the phase drop across a Josephson junction in this material.
31 Oct 01:42

A gate-tunable graphene Josephson parametric amplifier

by Guilliam Butseraen

Nature Nanotechnology, Published online: 24 October 2022; doi:10.1038/s41565-022-01235-9

Parametric amplifiers enable the low noise readout of systems with intrinsically low energy scales. Now, a parametric amplifier leveraging a graphene Josephson junction exhibits a gate-tunable working frequency and a gain exceeding 20 dB with added noise close to the standard quantum limit.
31 Oct 01:42

Continuous epitaxy of single-crystal graphite films by isothermal carbon diffusion through nickel

by Zhibin Zhang

Nature Nanotechnology, Published online: 27 October 2022; doi:10.1038/s41565-022-01230-0

Isothermal dissolution–diffusion–precipitation of carbon drives continuous epitaxial growth of single-crystal multilayer graphene.
31 Oct 01:42

Quantum-noise-limited microwave amplification using a graphene Josephson junction

by Joydip Sarkar

Nature Nanotechnology, Published online: 29 October 2022; doi:10.1038/s41565-022-01223-z

Low-noise amplification of feeble microwave signals is essential for superconducting quantum circuitry. Now, a gate-tunable Josephson parametric amplifier made from graphene shows 24 dB amplification paired with 10 MHz bandwidth and –130 dBm saturation power.
31 Oct 01:41

Electride surface hosts Wigner-crystal melting

by Atsushi Fujimori

Nature Materials, Published online: 25 October 2022; doi:10.1038/s41563-022-01382-3

Two-dimensional electrons on the surface of an electride are found to exhibit a phase transition from a normal Fermi liquid to an interesting quantum liquid, which is probably a quantum version of an electronic crystal beyond the melting point.
31 Oct 01:41

Twisted growth by design

by Seong-Jun Yang

Nature Materials, Published online: 25 October 2022; doi:10.1038/s41563-022-01378-z

Twisted bilayer graphene is epitaxially grown between two adjacent Cu(111) surfaces, with the twist angle controlled by the rotation of the Cu foils as designed.
31 Oct 01:41

Crossover from Ising- to Rashba-type superconductivity in epitaxial Bi2Se3/monolayer NbSe2 heterostructures

by Hemian Yi

Nature Materials, Published online: 27 October 2022; doi:10.1038/s41563-022-01386-z

Using molecular-beam epitaxy, we synthesize heterostructures of topological insulator Bi2Se3 and the Ising superconductor monolayer NbSe2. By changing the Bi2Se3 thickness, they demonstrate a crossover from Ising- to Rashba-type superconducting pairing.
31 Oct 01:41

Two-dimensional devices and integration towards the silicon lines

by Shuiyuan Wang

Nature Materials, Published online: 25 October 2022; doi:10.1038/s41563-022-01383-2

This Review discusses the progress in and potential pathways for incorporating two-dimensional materials into silicon platforms, from integrated devices to monolithic circuits.
31 Oct 01:37

Intrinsic glassy-metallic transport in an amorphous coordination polymer

by Jiaze Xie

Nature, Published online: 26 October 2022; doi:10.1038/s41586-022-05261-4

An unusual new material, NiTTFtt, is reported that is structurally amorphous, precluding a classical band structure, but detailed characterization reveals high conductivity and a metallic character.
24 Oct 01:40

Room‐Temperature Magnetic Skyrmions and Large Topological Hall Effect in Chromium Telluride Engineered by Self‐Intercalation

by Chenhui Zhang, Chen Liu, Junwei Zhang, Youyou Yuan, Yan Wen, Yan Li, Dongxing Zheng, Qiang Zhang, Zhipeng Hou, Gen Yin, Kai Liu, Yong Peng, Xi‐Xiang Zhang
Room-Temperature Magnetic Skyrmions and Large Topological Hall Effect in Chromium Telluride Engineered by Self-Intercalation

Magnetic skyrmions and large topological Hall effect are demonstrated in chromium telluride. The Curie temperature and magnetic anisotropy in Cr1+ x Te2 can be controlled by the self-intercalate concentration x. In Cr1.53Te2, which has a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy, room-temperature skyrmions and topological Hall resistivity as large as ≈106 nΩ cm are observed.


Abstract

Room-temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano-spintronic devices. However, such skyrmion-hosting materials are rare in nature. In this study, a self-intercalated transition metal dichalcogenide Cr1+ x Te2 with a layered crystal structure that hosts room-temperature skyrmions and exhibits large THE is reported. By tuning the self-intercalate concentration, a monotonic control of Curie temperature from 169 to 333 K and a magnetic anisotropy transition from out-of-plane to the in-plane configuration are achieved. Based on the intercalation engineering, room-temperature skyrmions are successfully created in Cr1.53Te2 with a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy. Remarkably, a skyrmion-induced topological Hall resistivity as large as ≈106 nΩ cm is observed at 290 K. Moreover, a sign reversal of THE is also found at low temperatures, which can be ascribed to other topological spin textures having an opposite topological charge to that of the skyrmions. Therefore, chromium telluride can be a new paradigm of the skyrmion material family with promising prospects for future device applications.

24 Oct 01:36

[ASAP] Multidimensional Building Blocks for Molecular Sieve Membranes

by Yujie Ban and Weishen Yang

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Accounts of Chemical Research
DOI: 10.1021/acs.accounts.2c00434
24 Oct 01:35

[ASAP] Thickness- and Twist-Angle-Dependent Interlayer Excitons in Metal Monochalcogenide Heterostructures

by Wenkai Zheng, Li Xiang, Felipe A. de Quesada, Mathias Augustin, Zhengguang Lu, Matthew Wilson, Aditya Sood, Fengcheng Wu, Dmitry Shcherbakov, Shahriar Memaran, Ryan E. Baumbach, Gregory T. McCandless◇, Julia Y. Chan◇, Song Liu, James H. Edgar, Chun Ning Lau, Chun Hung Lui, Elton J. G. Santos, Aaron Lindenberg, Dmitry Smirnov, and Luis Balicas

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ACS Nano
DOI: 10.1021/acsnano.2c07394
24 Oct 01:35

[ASAP] Magnetotransport in Graphene/Pb0.24Sn0.76Te Heterostructures: Finding a Way to Avoid Catastrophe

by Gregory M. Stephen, Ivan Naumov, Nicholas A. Blumenschein, Y.-J. Leo Sun, Jennifer E. DeMell, Sharmila N. Shirodkar, Pratibha Dev, Patrick J. Taylor, Jeremy T. Robinson, Paul M. Campbell, Aubrey T. Hanbicki, and Adam L. Friedman

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ACS Nano
DOI: 10.1021/acsnano.2c08911
24 Oct 01:35

[ASAP] Plasmonic-Thermoelectric Nanotweezers for Immersive SERS Mapping

by Xianyou Wang, Yuquan Zhang, Jiahao Yu, Xi Xie, Ruping Deng, Changjun Min, and Xiaocong Yuan

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ACS Nano
DOI: 10.1021/acsnano.2c07103
24 Oct 01:33

[ASAP] Co-Ion Desorption as the Main Charging Mechanism in Metallic 1T-MoS2 Supercapacitors

by Sheng Bi and Mathieu Salanne

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ACS Nano
DOI: 10.1021/acsnano.2c07272
24 Oct 01:18

Excitonic resonances control the temporal dynamics of nonlinear optical wave mixing in monolayer semiconductors

by Jonas M. Bauer

Nature Photonics, Published online: 17 October 2022; doi:10.1038/s41566-022-01080-1

Researchers show that resonant coupling of light pulses with excitonic transitions affects the optimal time difference between pulses for sum-frequency generation and four-wave mixing in monolayer WSe2.
24 Oct 01:18

A general one-step plug-and-probe approach to top-gated transistors for rapidly probing delicate electronic materials

by Laiyuan Wang

Nature Nanotechnology, Published online: 20 October 2022; doi:10.1038/s41565-022-01221-1

A one-step simultaneous van der Waals integration of high-k dielectrics and contacts enables the realization of top-gated transistors with atomically clean and electronically sharp interfaces.
17 Oct 01:17

An optoelectronic synapse based on α-In2Se3 with controllable temporal dynamics for multimode and multiscale reservoir computing

by Keqin Liu

Nature Electronics, Published online: 13 October 2022; doi:10.1038/s41928-022-00847-2

A reservoir computing system for multimode and multiscale signal processing can be created using optoelectronic synapses that are based on α-In2Se3 and exploit the tightly coupled ferroelectric and optoelectronic properties of the material.
17 Oct 01:04

Tailored Ising superconductivity in intercalated bulk NbSe2

by Haoxiong Zhang

Nature Physics, Published online: 13 October 2022; doi:10.1038/s41567-022-01778-7

The superconducting critical temperature of monolayer materials is often lower than their bulk counterparts. Now, intercalation is shown to induce two-dimensional superconducting properties while maintaining the bulk critical temperature.